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Progress in Chemistry 2012, Vol. Issue (9): 1801-1817 Previous Articles   Next Articles

• Review •

Catalysts for Catalytic Decomposition of Nitrous Oxide

Li Mengli1,2, Yang Xiaolong1, Tang Liping1,2, Xiong Xumao1, Ren Sili1, Hu Bin1   

  1. 1. Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China;
    2. Graduate University of Chinese Academy of Sciences, Beijing 100049, China
  • Received: Revised: Online: Published:
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Nitrous oxide(N2O)originating from industrial and automotive emissions is accepted to be a major air pollutant. It contributes to the greenhouse effect and the depletion of stratospheric ozone. In recent years, elimination of N2O has attracted increasing attention for concerns from environment pollution. The necessity to reduce N2O emissions requires the development of catalytic technologies. Direct catalytic decomposition of N2O to N2 and O2 has been recognized as one of the most prospect methods for elimination pollution derived from N2O, since it does not require the addition of any reductant, without causing secondary pollution, and the process it concerned is simple and economical. This paper reviews the advance of several interesting catalysts that have been paid great attention in recent years, including metal oxides, noble metals and ion-exchanged zeolites catalyst systems. The advantages and disadvantages of the catalysts are also discussed in detail. This review also covers the research progress of reaction mechanism, molecular simulation and reaction kinetics on the surface of solid catalysts. Besides, the effects of moecular oxygen, water, sulfur dioxide and other species on the catalysts' activity, life and stability, are also included in this paper. The demerits exist both in these catalysts and theoretical research for the decomposition of N2O are pointed out. Finally, the trends in the catalyst system for direct catalytic decomposition of N2O are prospected. Contents 1 Introducion
2 Catalysts
2.1 Metal oxides
2.2 Noble metals
2.3 Ion-exchange zeolites
3 Reaction mechanism, molecular simulation and reaction kinetics
3.1 Reaction mechanism
3.2 Molecular simulation
3.3 Reaction kenetics
4 The effection caused by other speices
4.1 The effect of NOx
4.2 The effect of O2
4.3 The effect of H2O
4.4 The effect of SO2
4.5 The effect of reductant
5 Conclusion and outlook
Key words: nitrous oxide, catalytic decomposition, reaction mechanism, inhibition effect, poisoning effect

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