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Progress in Chemistry 2023, Vol. 35 Issue (7): 1018-1029 DOI: 10.7536/PC221203 Previous Articles   Next Articles

• Review •

Interactions Between Humic Acid and Co-Existing Substances in Aquatic Environments

Chundi Zhou1, Minghao Sui1,2()   

  1. 1 State Key Laboratory of Pollution Control and Resource Reuse, College of Environmental Science and Engineering, Tongji University,Shanghai 200092, China
    2 Shanghai Institute of Pollution Control and Ecological Security,Shanghai 200092, China
  • Received: Revised: Online: Published:
  • Contact: * e-mail: suiminghao.sui@gmail.com
  • Supported by:
    National Key R&D Program of China(2019YFC0408801)
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Humic acid (HA) has attracted significant attention in the field of environmental remediation due to its occurrence characteristics and unique chemical reactivity. It is worth noting that in co-existing reaction systems, HA inevitably interacts with co-existing substances, making the reaction system complex and leading to unexpected results. Therefore, studying the interaction between HA and co-existing substances is of great significance for a correct understanding of the complexity of environmental water pollution and the development of new environmental functional materials with cooperative treatment of co-existing substances. This article reviews the synergistic/antagonistic removal effects of target pollutants in co-existing pollution systems involving HA, including inorganic co-existing pollutant systems, organic co-existing pollutant systems, and microbial co-existing systems. Based on the structural characteristics and physicochemical properties of HA itself, the interaction mechanisms between HA and co-existing pollutants are systematically analyzed. These mechanisms mainly involve coordination, electrostatic interactions, adsorption, hydrophobic interactions, π-π interactions, and oxidation-reduction reaction (REDOX). Finally, the challenges and future research directions for the removal of target pollutants by HA in co-existing pollution systems are discussed.

Contents

1 Introduction

2 Removal of target contaminant in different co-existing systems

2.1 HA with co-inorganic contaminant system

2.2 HA with co-organic contaminant system

2.3 HA with co-microbial system

2.4 Quantitative comparison of the removal effectiveness in HA co-existing contaminant systems

3 Interaction mechanisms between HA and co-existing contaminant

3.1 HA with co-inorganic contaminant system

3.2 HA with co-organic contaminant system

3.3 HA with co-microbial system

3.4 Characteristics of interaction mechanism in HA co-existing contaminant systems

4 Conclusion and Outlook

Key words: humic acid, environmental water pollution, co-existing substances, interaction, co-existing systems
Fig.1 Structural units and functional groups of HA[8] Copyright 2011, Springer Nature
Fig.2 The removal synergistic or antagonistic effect of contaminants with HA in co-existing system
Table 1 Standard redox potential of heavy metal ions
Cr
(Ⅵ)		 Fe
(Ⅲ)		 Pb
(Ⅱ)		 Cd
(Ⅱ)		 Mg
(Ⅱ)		 Na
(Ⅰ)		 Ca
(Ⅱ)		 K
(Ⅰ)
E0 (Ⅴ) 1.33 0.77 -0.13 -0.40 -2.37 -2.71 -2.87 -2.93
Fig.3 The possible mechanism of high-dispersion zero-valent iron particles stabilized by artificial humic acid for lead ion removal[70]. Copyright 2019, Elsevier
Fig.4 The possible mechanism of transformation of silver ions to silver nanoparticles mediated by humic acid under dark conditions[92]. Copyright 2019, Elsevier
Fig.5 Schematic diagram of the possible mechanism of HA affecting the adsorption of THIA on MPFs[101]. Copyright 2022, Elsevier
Fig.6 Potential mechanism of Gt-HA promoted Fenton-like degradation of SA[61]. Copyright 2020, Elsevier
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