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Progress in Chemistry 2012, Vol. Issue (9): 1683-1695 Previous Articles   Next Articles

• Review •

Structure and Supramolecuclar Properties of Arylacetylene Macrocycles

Li Jie, Huang Pengcheng   

  1. School of Materials Science and Engineering, Beihang University, Beijing 100191, China
  • Received: Revised: Online: Published:
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Arylacetylene macrocycles (AEMs) that contain shape-persistent backbones and allow the attachment of (functional) side groups at defined positions have attracted much attention since their invention. Due to the large π-conjugated system and the flexible bonding points at the ring, arylacetylene macrocycles are especially valuable candidates for the construction of complex supramolecular architectures. This review covers the recent progress in the research on the supramolecular properties of arylacetylene macrocycles, including aggregation in solution, liquid crystal behavior, one-dimensional self-assembly and supramolecular-assembled monolayer at the substrate surface or at the solid-liquid interface. The investigation method is introduced. The relationship between the molecular structure and the supramolecular property of AEMs are elaborated, and potential applications of AEMs are indicated. It will be helpful for the preparation of novel materials with desired size, shape and functionality through rational molecular design. Contents 1 Introduction
2 Aggregation of arylacetylene macrocycles in solution
3 Liquid crystal behavior of arylacetylene macrocycles
3.1 Nematic liquid crystal
3.2 Columnar liquid crystal
4 One-dimensional self-assembly of arylacetylene macrocycles
4.1 Influence of molecular structure
4.2 Influence of fabrication conditions
5 Monolayer of arylacetylene macrocycles at the substrate surface or at the solid-liquid interface
5.1 Influence of molecular structure
5.2 Influence of solvent and substrate
5.3 Influence of guest molecule
6 Conclusion and outlook
Key words: arylacetylene macrocycle, molecular structures, supramolecular properties, self-assembly

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