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Progress in Chemistry 2009, Vol. 21 Issue (09): 1869-1879 Previous Articles   Next Articles

• Review •

Polymerization in Surpercritical Carbon Dioxide

Zhang Huaiping1**|Chen Mingcai   

  1. (1.College of Materials Science and Engineering, Taiyuan University of Technology, Taiyuan 030024, China|2.Guangzhou Institute of Chemistry, Chinese Academy of Sciences, Guangzhou 510650, China)
  • Received: Revised: Online: Published:
  • Contact: Zhang Huaiping E-mail:huaipingzhang@gmail.com
  • Supported by:

    National Natural Science Foundation of China

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The recent progress of polymerization in supercritical carbon dioxide is reviewed. The advantage of supercritical carbon dioxide used as an environmental medium in polymerization and reactions in supercritical carbon dioxide are described. It includes homogeneous free radical polymerizations, precipitation free radical polymerizations, dispersion free radical polymerizations, emulsion and inverse emulsion free radical polymerizations, cationic polymerizations, ring-opening polymerization, melt-phase condensation polymerizations, sol-gel polymerizations, polymer blend synthesis, catalytic chain transfer polymerizations, oxidative coupling polymerization, nitroxide-mediated radical dispersion, atom-transfer radical polymerization, reversible addition-fragmentation chain transfer polymerization, electrochemical polymerization, simultaneous one-pot combination of enzymatic and chemical polymerization, copolymerization of carbon dioxide used as monomer.

Contents
1 Introduction
2 Free-radical polymerizations
2.1 Homogeneous polymerizations
2.2 Precipitation polymerizations
2.3 Dispersion and emulsion polymerizations
2.4 Inverse emulsion and pseudo dispersion polymerizations
2.5 Polymer blend synthesis
3 Cationic polymerizations
4 Step-growth polymerizations
4.1 Melt-phase condensation polymerizations
4.2 Oxidative coupling polymerization
4.3 Sol-gel polymerizations
5 Living polymerizations
5.1 Reversible addition-fragmentation chain transfer polymerization
5.2 Nitroxide-mediated radical dispersion
5.3 Atom-transfer radical polymerization
6 Other polymerizations
6.1 Ring-opening polymerization
6.2 Catalytic chain transfer polymerizations
6.3 Electrochemical polymerization
6.4 Hydrosilation polymerization
6.5 Simultaneous one-pot combination of enzymatic and chemical polymerization
6.6 CO2 copolymerization
7 Outlook

Key words: supercritical fluid, supercritical carbon dioxide(ScCO2), polymerization

CLC Number: 

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