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Progress in Chemistry 2008, Vol. 20 Issue (10): 1453-1464 Previous Articles   Next Articles

• Review •

Low-temperature Catalytic Oxidation of Carbon Monoxide

Liang Feixue1,2 Zhu Huaqing1 Qin Zhangfen1 Wang Guofu1 Wang Jianguo1**

  

  1. (1. State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China;
    2. Graduate School of Chinese Academy of Sciences, Beijing 100049, China)
  • Received: Revised: Online: Published:
  • Contact: Wang Jianguo
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The catalytic oxidation of carbon monoxide (CO) at low temperature has attracted considerable attention because of its wide applications in exhaust abatement for CO2 lasers, trace CO removal in enclosed atmospheres, automotive emission control, and CO preferential oxidation (PROX) for proton exchange membrane fuel cells (PEMFC). Progress in low-temperature catalytic oxidation of CO is summarized. Catalysts and preparation method, reaction mechanisms of CO oxidation and the effects of different coexisted atmospheres on the catalytic performance of the catalysts are reviewed. The preparation methods include impregnation, coprecipitation, deposition-precipitation, sol-gel, ion exchange, chemical vapor deposition, electrochemistry deposition, inert gases condensation, and solvated metal atom impregnation so on. The catalysts for low-temperature CO oxidation consist of noble metal catalysts, non-noble metal catalysts, catalysts supported on molecular sieves and alloy catalysts. The mechanisms on low-temperature CO oxidation are reported by many researchers, and plentiful hypothesises are put forward on different catalysts. The effect of H2O, CO2, H2 and many other coreactants on the performance of low-temperature are expatiated on. The prospects for this field are brought forward at last.
Key words: CO oxidation, PROX, low-temperature, catalysts, mechanisms

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