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Progress in Chemistry 2007, Vol. 19 Issue (01): 6-34 Previous Articles   Next Articles

• Special issues •

A New Era for Organic Synthesis Highlights of the Recent Progress

Wu Yikang;Wu Yulin   

  1. State Key Laboratory of Biooraganic and Natural Products Chemistry,Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences,Shanghai 200032
  • Received: Revised: Online: Published:
  • Contact: Wu Yikang;Wu Yulin
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The major progress in organic synthesis since 2005 is briefly surveyed in two parts. The first part deals with some of the most impressive advances in the synthetic methodology, which includes: (1) Metal-mediated synthetic reactions, with an emphasis on the olefin metathesis and gold-mediated reactions. (2) Free radical-based organic synthesis. (3) Synthetic transformations performed in a 'one-pot' manner involving either tandem reactions or multi-component reactions. (4) Asymmetric reactions catalyzed by metal and organo-catalysts. The major advances in total synthesis of some complex natural products with significant biological activities are presented in the second part, with detailed illustrations of 10 selected molecules, including dragmacidin F, abyssomisin C, 11-acetoxy-4-deoxyasbestinin D, pentacycloanammoxic acid, UCS1025A, (-)-Merrilactone A, nigellamine A2, (+)-saxitoxin, and tamiflu (an artificially designed natural-like molecule). An array of complicated structures of the natural products synthesized over the last two years are also listed to serve as a convenient lead to the original literature for the prospective interested readers.
Key words: organic synthesis, metal-mediated synthetic reaction, free radical reaction, in one potreaction, asymmetric reaction, total synthesis of natural products

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