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Progress in Chemistry 2003, Vol. 15 Issue (01): 51- Previous Articles   Next Articles

• Review •

Catalytic Oxidation of Benzene to Phenol by FeZSM-5/N2O

Ji Dong;Ren Tong;Zhang Xiaoming;Suo Jishuan*;Ding Yong   

  1. ( State Key Laboratory for Oxo Synthesis and Selective Oxidation,Lanzhou Institute of Chemical Physics,Chinese Academyof Sciences, Lanzhou 730000, China)
  • Received: Revised: Online: Published:
  • Contact: Suo Jishuan
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One step oxidation of benzene to phenol has been a challenging subject in organic synthesis.In this review,the focus is on the recent advances in gas-phase catalytic oxidation over zeolites using nitrous oxide as oxidant.The remarkbleness of this catalyst system lies in catalytic α-oxygen that is got from N2O decomposed over zeolites.The specific structure of Fe-containing active sites and the mechanism of the reaction were considered. This process of one step oxidation of phenol over FeZSM-5/N2O seems to be quite promising and promotes the development of new ecologically safe technologies for organic synthesis.
Key words: zelites, dinitrogen monoxide, phenol synthesis, selective catalytic oxidation, FeZSM-5

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