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Progress in Chemistry DOI: 10.7536/PC231023   

Study on the High-Voltage Resistance of Layered Oxide Cathode Materials for Sodium-ion Batteries

Lixiang Ding, Xuke Li, Xuefeng Liu, Yimin Liu, Wen Lei*, Haijun Zhang*   

  1. The State Key Laboratory of Refractories and Metallurgy, Wuhan University of Science and Technology, Wuhan 430081, China
  • Received: Revised:
  • Contact: *e-mail: leiwen@wust.edu.cn.（Wen Lei）;zhanghaijun@wust.edu.cn(Haijun Zhang)
  • Supported by:
    National Natural Science Foundation of China (No. 52072274, 52272021, 52232002), the Knowledge Innovation Project of Wuhan, China (2023020201010131).
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Sodium-ion batteries have shown great application prospects in the field of large-scale energy storage and low-speed electric vehicles due to their resource and cost advantages. Among various cathodes reported, layered oxide cathode materials have been widely investigated owing to their high theoretical capacity and simple synthesis method. However, many adverse reactions and phenomena such as structural instability and surface degeneration are prone to occur during its cycling process, especially at high voltage, which hinders its application in commerce. This article briefly reviews the mechanism of structural transformation, surface degradation, and oxygen loss of layered oxide cathode at high-voltage, focuses on the strategies to improve the high-pressure resistance of layered oxide cathode, and aims to provide reasonable insights for improving the high-voltage stabilization of layered oxide cathode materials and designing sodium-ion layered oxide cathode materials with high performance. Finally, the shortcomings of sodium battery layered oxide cathode materials in modification and future research directions are also summarized.
Key words: sodium-ion battery, layered oxide, cathode materials, high-voltage performance
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