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Progress in Chemistry 2023, Vol. 35 Issue (10): 1544-1558 DOI: 10.7536/PC230215 Previous Articles   

• Review •

Application of Pyrite and Its Modified Composite in Water Pollution Treatment

Yanxiao Chi1, Yuxuan Yang1, Kunlun Yang1,2,*(), Xianrong Meng2, Wei Xu2, Hengfeng Miao1   

  1. 1 College of Environment and Civil Engineering, Jiangnan University,Wuxi 214122, China
    2 Suzhou Institute of Environmental Science, Jiangsu Postdoctoral Innovation Practice Base,Suzhou 215009
  • Received: Revised: Online: Published:
  • Contact: *e-mail: yangkunlun@jiangnan.edu.cn
  • Supported by:
    National Natural Science Foundation of China(22206061); Fundamental Research Funds for the Central Universities(JUSRP122022)
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Due to its strong surface activity, precipitation adsorption, redox and relatively excellent photocatalytic properties, pyrite has been widely used to treat heavy metals, organic pollutants and various inorganic salts in the polluted water. However, some inherent defects of pyrite, such as small specific surface area, high susceptibility to agglomeration, etc., limit its practical applications. Appropriate modification of pyrite via morphological adjustment, elemental doping, and material loading can improve the dispersion performance of particle size, expose more functional groups and increase electron transport rate to further modulate the related properties and enhance the wastewater treatment capacity of pyrite, In this article, we firstly introduce the basic information, the application and the mechanism of pyrite in wastewater treatment, and then describe the typical modification methods of pyrite and their corresponding strengthening mechanisms for treating wastewater. This article will provide a systematic introduction and outlook for the development of pyrite-based composite materials in the field of environmental treatment.

Contents

1 Introduction

2 Adsorption of pyrite

2.1 Application and mechanism of pyrite adsorption capacity

2.2 Improvement of pyrite materials and enhancement of adsorption capacity

3 Oxidation of pyrite

3.1 Application and mechanism of pyrite oxidation ability

3.2 Improvement of pyrite materials and enhancement of oxidation capacity

4 Reduction of pyrite

4.1 Application and mechanism of pyrite reduction ability

4.2 Improvement of pyrite materials and enhancement of reduction capacity

5 Conclusion and outlook

Key words: pyrite, modification, functional regulation, water pollution treatment
Fig.1 Crystal structure of pyrite[10]
Fig.2 Mechanism of pyrite adsorbing heavy metals[25]
Fig.3 Mechanism of pyrite adsorbing organic pollutants
Fig.4 Some typical strategies to enhance the adsorption performance of pyrite for the removal of heavy metals
Table 1 Adsorption and removal of heavy metals by pyrite modified materials
Modification method Modification material Target metal Removal performance ref
Ball-milling BM-ZVI/FeS2 Sb(V) 134 mg/g 20
BM-FeS2 Pb(Ⅱ) 34.10 mg/g 42
BM-FeS2 Cr(Ⅵ),Cd(Ⅱ),Pb(Ⅱ) 4.75 mg/g, 2.87 mg/g, 4.91 mg/g 46
Thermal modification SV-FeS2 Ni(Ⅱ) 6.45 mg/g 21
FeS2/α-Fe2O3 Sb(V) 347.2 mg/g 43
Element doping Ni-FeS2 Se(Ⅳ) 15.79 mg/g 44
Loading PY+AC-FA Hg(Ⅱ) 239.26 μg/g 45
Fig.5 Mechanism of heavy metal removal by pyrite oxidation
Fig.6 Proposed mechanisms of pyrite-mediated Fenton oxidation and persulfate oxidation processes for the degradation of organic pollutants[4]
Table 2 Removal of heavy metals by oxidation of pyrite modified materials
Modification method Modification material Target metal Removal performance ref
Surface oxidized surface-oxidized pyrite Sb(Ⅲ) 0.4 mg/g 73
Enhanced oxidation Fe2++FeS2 As(Ⅲ) 10 mg/g 70
FeS2 + PMS As(Ⅲ) 5 mg/g 74
FeS2+UV As(Ⅲ) 13.3 mg/g 72
Loading Fe0/FeS2 As(Ⅲ) 1 mg/g 75
FeS2/NaClO As(Ⅲ) 2.5 mg/g 76
Table 3 Modified pyrite catalytic oxidation degradation of organic compounds
Modification method Modification material Target metal Removal performance ref
Ball-milling Pyrite nanoparticles Acid orange 7 16 mg/g 77
nano-pyrite Sulfadiazine 10 mg/g 82
Heterostructure FeS2/Fe2O3+TA Carbamazepine 1.3 mg/g 78
TiO2/FeS2 Methylene blue 6.1 mg/g 83
Fe3O4@FeS2@C@MoS2 Tetracycline 12.5 mg/g 84
ZnCo2O4/MnO2/FeS2 Methyl orange 3.84 mg/g 85
FeS2/rGO Methylene blue 41.67 mg/g 86
FeS2-Fe1-xS Acid orange 7 15 mg/g 87
CuO-FeS2 Brilliant green 2 mg/g 88
Loading FeS2/H2O2+AC, BC, CNTS Ciprofloxacin 89 mg/g, 71 mg/g, 68 mg/g 80
Fig.7 Mechanism of Cr(Ⅵ) reduction by pyrite[91]
Fig.8 Mechanism of reduction of non-metallic ions by pyrite
Fig.9 Reaction mechanism of pyrite reducing organic pollutants
Table 4 Removal of heavy metals by reduction with pyrite modified materials
Modification method Modification material Target metal Removal performance ref
Ball-milling BM-FeS2@BC Cr(Ⅵ) 134 mg/g 103
Element doping Ni-FeS2/FeS2 Cr(Ⅵ) 40 mg/g 104
Heterostructure FeS2/Fe2O3 Cr(Ⅵ) 37.5 mg/g 6
α-FeOOH/FeS2 Cr(Ⅵ) 25 mg/g 105
Loading FeS2+Sepiolite Cr(Ⅵ) 14.27 mg/g 102
FeS2/Fe0 Cr(Ⅵ) 16.67 mg/g 106
FeS2/biochar Cr(Ⅵ) 10 mg/g 107
pyrite-marcasite-magnetite Cr(Ⅵ) 50 mg/g 108
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