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Progress in Chemistry 2022, Vol. 34 Issue (4): 950-962 DOI: 10.7536/PC210442 Previous Articles   Next Articles

• Review •

Construction of Magnetic NiFe2O4-Based Composite Materials and Their Applications in Photocatalysis

Xiaowei Li1, Lei Zhang2(), Qixin Xing1, Jinyu Zan1, Jin Zhou1, Shuping Zhuo1   

  1. 1 School of Chemistry and Chemical Engineering, Shandong University of Technology,Zibo 255000, China
    2 School of Materials Science and Engineering, Anhui University of Science and Technology,Huainan 232001, China
  • Received: Revised: Online: Published:
  • Contact: Lei Zhang
  • Supported by:
    National Natural Science Foundation of China(51502162); National Natural Science Foundation of China(21975001); Key Project of Natural Science Research for Colleges and Universities of Anhui Province of China(KJ2019A0115); Young Teacher Supporting Fund of Shandong University of Technology
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Environmental pollution and energy shortage caused by the rapid development of the economy have become two major problems in modern society. Accordingly, much research is currently focused on the exploitation of new alternative energy sources. Among various energy sources, solar energy is considered to be ideal and renewable energy. Under sunlight irradiation, photocatalysis, as a novel “green technology”, can directly convert organic pollutants into innoxious substances to solve both energy crisis and environmental pollution. However, the key to the success of this process is dependent on the rational design and fabrication of efficient photocatalysts. The NiFe2O4 possessing fast magnetism response and good photochemistry stability, is coupled with other semiconductor photocatalysts having a suited band gap in order to obtain greatly effective photocatalytic systems and achieve the magnetic separation, exhibiting wide application foreground. This paper mainly reviews the latest research progress on the synthesis and photocatalytic application of NiFe2O4-based composites, which may open a new avenue and idea for preparing highly active and magnetically separable composite photocatalysts. Finally, the future development of NiFe2O4-based photocatalytic materials is also prospected.

Contents

1 Introduction

2 NiFe2O4/carbon materials

2.1 NiFe2O4/graphene

2.2 NiFe2O4/g-C3N4

2.3 NiFe2O4/other carbon materials

3 NiFe2O4/Bismuth-based compounds

3.1 NiFe2O4/BiOX

3.2 NiFe2O4/Aurivillius Bismuth-based oxide

3.3 NiFe2O4/other Bismuth-based compounds

4 NiFe2O4/Silver-based compounds

4.1 NiFe2O4/Ag3PO4

4.2 NiFe2O4/AgX

5 NiFe2O4/TiO2

6 NiFe2O4/ZnO

7 Conclusion and outlook

Key words: NiFe2O4, magnetic, composites, photocatalysis
Fig. 1 Mechanism of photocatalytic degradation of MB in the presence of NiFe2O4-RGO[24]
Fig. 2 The proposed direct Z-scheme photocatalytic mechanism for the g-C3N4/NiFe2O4 nanocomposite[35]
Fig. 3 The proposed all-solid-state Z-scheme photocatalytic mechanism for the g-C3N4/graphene/NiFe2O4 nanocomposite[39]
Fig. 4 (a,b) SEM images,(c) TEM image and (d) HRTEM image of NiFe2O4/C[40]
Table 1 The photocatalytic activity of pollutant degradation over different NiFe2O4/carbon material composites
Photocatalyst Pollutant Degradation efficiency (%) Degradation
time(min)		 Light condition ref
NiFe2O4-RGO Methylene blue 20 mg/L ~99.1 180 800 W Xe lamp, visible light 24
NiFe2O4@GO Methylene blue 0.04 mmol/L ~100 120 10 W UV lamp, UV light 25
2%NiFe2O4/g-C3N4 Methyl orange 10 mg/L ~68 60 300 W Xe lamp, visible light 33
NiFe2O4-g-C3N4 Methylene blue 20 mg/L ~98 225 40 W LED bulb, visible light 34
NiFe2O4-g-C3N4 Rhodamine B 10 mg/L ~90 225 40 W LED bulb, visible light 34
NiFe2O4-g-C3N4 Methylene blue 20 mg/L ~99 225 direct sunlight 34
NiFe2O4-g-C3N4 Rhodamine B 10 mg/L ~99 225 direct sunlight 34
g-C3N4/NiFe2O4 Methyl orange 10 mg/L ~100 210 10 W LED lamp, visible light 35
g-C3N4/NiFe2O4-12% Methylene blue 50 mg/L ~100 75 300 W Xe lamp, visible light 36
Boron doped g-C3N4/NiFe2O4 Methylene blue 5 mg/L ~98 80 350 W Mercury-Xenon lamp 37
20%NiFe2O4@P-g-C3N4 Phenol 20 mg/L ~96 60 Direct sunlight 38
20%NiFe2O4@P-g-C3N4 Hydrogen production ~904 μmol/h 150 W Xe arc lamp, visible light 38
g-C3N4/graphene/NiFe2O4-25% Methyl orange 10 mg/L ~100 120 10 W LED lamp, visible light 39
NiFe2O4/C Tetracycline hydro chloride 20 mg/L ~97.25 60 800 W Xe lamp, visible light 40
25%NiFe2O4-MWCNT Sulfamethoxazole 5 mg/L ~100 120 100 W mercury lamp, UV-A light 41
Fig. 5 (a,b) TEM images of NiFe2O4/BiOBr[53]
Fig. 6 (a) TEM image of NiFe2O4/BiOBr; (b) HRTEM image of NiFe2O4/BiOBr[54]
Fig. 7 Band structure and possible photogenerated charges migration path of NiFe2O4/BiOI nanocomposite[56]
Fig. 8 Photocatalytic mechanism of MB degradation by Ag3PO4/Ag/NiFe2O4 composite[81]
Fig. 9 (a,b) SEM images of Ag3PO4/GO/NiFe2 O4[82]
Fig. 10 Photocatalytic mechanism of Ag3PO4/GO/NiFe2O4 composite[82]
Fig. 11 Photocatalytic mechanism of AFO/MOF/NFO[84]
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