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Progress in Chemistry 2020, Vol. 32 Issue (2/3): 274-285 DOI: 10.7536/PC190602 Previous Articles   Next Articles

Two-Dimensional Covalent Organic Frameworks Photocatalysts

Suyan Zhao1, Chang Liu2, Hao Xu3, Xiaobo Yang2,**()   

  1. 1. Jilin Police College, Changchun 130117, China
    2. College of Chemistry and Chemical Engineering, Shenyang Normal University, Shenyang 110034, China
    3. College of Chemistry and Chemical Engineering, Henan University, Kaifeng 475004, China
  • Received: Online: Published:
  • Contact: Xiaobo Yang
  • About author:
    ** e-mail: ;
  • Supported by:
    National Natural Science Foundation of China(21806167); Natural Science Foundation of Liaoning Province(20180550882); Innovation and Entrepreneurship Training Program for College Students(201910076)
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Two-dimensional Covalent organic frameworks(2D-COFs), as a new type of crystalline porous materials constructed with organic building blocks, possessing regular pore structure, good stability, high surface area and extended π-conjugation system, have shown good photoactivity and tremendous potential for light-driven chemical transformations. Therefore, the application of 2D-COFs in light-driven chemical transformations has recently garnered great attention in both porous materials science and photocatalysis. This review mainly summarizes and discusses the applications of photoactive 2D-COFs in light-driven chemical transformations in recent years. Future development is also prospected.

Key words: two-dimensional covalent organic frameworks, photocatalyst, porous materials, light-driven chemical transformations, structure and property
Fig.1 The development of COFs[29, 34]
Fig.2 Synthetic routine for TFPT-COF
Fig.3 Transformation of TFPT-COF during photocatalysis and subsequent recovery by reconversion[44]
Fig.4 Synthesis of two-dimensional azine-linked N x -COFs
Fig.5 Optical and photocatalytic properties of N x -COFs[45]
Fig.6 The synthesis of diacetylene based COFs
Fig.7 Synthesis of CTFs photocatalyst via a polycondensation approach under mild conditions
Fig.8 Synthesis of highly crystalline CTFs photocatalyst
Fig.9 Light-driven conversion of CO2 catalyzed by 2D-COFs[52]
Fig.10 Proposed catalytic mechanism for CO2 reduction[53]
Fig.11 Synthesis of benzothiadiazole functionalized covalent organic frameworks[56]
Fig.12 Photoreduction of Cr(Ⅵ) by BT-COFs[56]
Fig.13 Synthesis of hydrazine-based 2D-COFs[64]
Fig.14 UV/Vis spectra of TFB-COF and its monomers[64]
Fig.15 TFB-COF catalyzed visible-light driven CDC reaction[64]
Fig.16 COF-JLU5 catalyzed visible-light driven CDC reaction[65]
Fig.17 Synthesis of LZU-190, LZU-191 and LZU-192[66]
Fig.18 Substrates compatibility for the reaction[66]
Fig.19 Proposal mechanism for the LZU-190 visible-light-driven oxidative hydroxylation[66]
Fig.20 Synthesis of COFs with benzothiadiazole and pyrene units[67]
Fig.21 UV/Vis diffuse reflection spectra and plot of Kubelda-Munk function for the band gap of COF-JLU22[67]
Fig.22 Proposal mechanism for the COF-JLU22 catalyzed photocatalytic debromination[67]
Fig.23 Visible-light-induced tandem radical addition-cyclization of 2-aryl phenyl isocyanides catalysed by recyclable covalent organic frameworks, 2D-COFs[75]
Fig.24 Optical and electrochemical properties of 2D-COF-1[75]
Fig.25 Proposed mechanism for the 2D-COF-1 catalyzed photocatalytic radical addition and cyclization[75]
Fig.26 Synthesis of a 2D porphyrin-based sp2 carbon conjugated COF[78]
Fig.27 Por-sp2c-COF catalyzed photocatalytic oxidation of secondary amines to imines[78]
Fig.28 TpTt catalyzed photocatalytic E-Z isomerization of olefins[79]
Fig.29 Photocatalytic crystalline laminar covalent organic framework for the oxidation of sulfides[80]
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