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Progress in Chemistry 2019, Vol. 31 Issue (8): 1177-1186 DOI: 10.7536/PC181215 Previous Articles   Next Articles

Nickel-Manganese Binary Metal Oxide as Electrode Materials for Supercapacitors

Shaoming Qiao, Naibao Huang**(), Zhengyuan Gao, Shixian Zhou, Yin Sun   

  1. College of Transportation Engineering, Dalian Maritime University, Dalian 116026, China
  • Received: Online: Published:
  • Contact: Naibao Huang
  • About author:
    ** E-mail:
  • Supported by:
    National Key Research and Development Program of China(2016YFB0101206); National Natural Science Foundation of China(21676040); National Natural Science Foundation of China(21276036); Dalian Science and Technology Innovation Funds(2018J12GX053)
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Pseudocapacitors have a higher specific capacitance than electrochemical double-layer capacitors (about 10~100 times). Since the Faraday reactions are simultaneously occur on the surface and inside of the electrode material during charging/discharging process. More electrons are generated and have a larger specific capacitance.At present, research on pseudocapacitance electrode materials mainly focuses on metal oxides and conductive polymers. Nickel-manganese-based metal oxides, as one of them, have the advantages of high theoretical specific capacitance, low cost, non-toxicity and environmental friendliness. However, its actual electrochemical performance is much lower than the theoretical value. Therefore, in order to improve the electrochemical performance of electrode materials. Some researchers have proposed many effective strategies, such as prepared of different kinds of metal oxides as electrode materials, use of different synthesis processes to prepare high specific surface area materials, the synergetic effect between the different materials and so on.In this paper, the application progress of nickel-manganese based binary metal oxides (NiMnO3, NiMn2O4 and Ni6MnO8) as pseudocapacitance electrode materials in supercapacitors has reviewed. At the same time, the future research directions of metal oxide electrode materials are further proposed.

Key words: supercapacitors, nickel-manganese based metal oxides, pseudocapacitors, electrode materials, high performance
Fig. 1 Sample preparation at different hydrothermal temperatures:(a)120,(b)140,(c)160, and (d)180 ℃[23]
Fig. 2 SEM images of(a) NiMnO3,(b) NiMnO3/Ni(OH)2,(c) Cyclic voltammetry curves and(d) galvanostatic discharge curves:1.NiMnO3/Ni(OH)2, 2.NiMnO3,3.MnOOH[27]
Fig. 3 (a) CV curves of all samples at the scan rate of 1 mV/s,(b) EIS of samples[35]
Fig. 4 (a)specific capacitance of NiMnO3 electrode material with different Fe ion mass ratios,(b)I-V plots of 15 wt% Fe-doped NiMnO3 and NiMnO3 powder[38]
Fig. 5 (a,b) SEM images of NiMn2O4 thin films[41]
Fig. 6 Porous sheets-like morphology NiMn2O4 material[42]
Fig. 7 (a) SEM image and(b) cycling performance of NiMn2O4 material[47]
Fig. 8 Characterization of the CNT@NiMn2O4 hybrid nanoarrays by SEM:(a) Low-magnification;(b) high-magnification;(c) TEM image;(d) TEM magnified images[52]
Fig. 9 SEM images of(a) Ni6MnO8,(b)NiO,(c)NiO/NMO-2,(d~f) Comparison of performance of different samples[73]
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