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Progress in Chemistry 2019, Vol. 31 Issue (7): 1056-1066 DOI: 10.7536/PC181212 Previous Articles   

The Preparation and Anti-Icing Properties of Flexible Surfaces

Cuiping Zhou1, Qiming Liu2, Xuan Zhao1, Chunsheng Li1, Hui Li1,**(), Shuxiang Zhang1,**()   

  1. 1.School of Chemistry and Chemical Engineering, Shandong Key Laboratory of Fluorine Chemistry and Chemical Engineering Materials, University of Jinan, Jinan 250022, China
    2.Shandong Institute of Construction and Development, Jinan 250001, China
  • Received: Online: Published:
  • Contact: Hui Li, Shuxiang Zhang
  • About author:
    ** E-mail: (Hui Li);
    (Shuxiang Zhang)
  • Supported by:
    Natural Science Foundation of Shandong Province(ZR2016EMM04); Natural Science Foundation of Shandong Province(ZR2017ZC0529); Natural Science Foundation of China(51103061)
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The attachment and accumulation of ice, a common natural phenomenon, brings many inconvenience and even serious disaster to human society. The anti-icing surface is a hot topic in current research, and the surface structure and properties of materials are the key factors that influence the icing. But up to date, there still exist some problems, such as poor stability and limitation of application conditions, to be further comprehensively and systematically studied due to the complexity of icing conditions and the diversity of icing types. In the review, based on the relationships between the anti-icing properties and the molecule’s flexibility or slippage of the material surface, the concept of the flexible anti-icing surface is proposed and the types and mechanisms of flexible anti-icing surfaces, including intrinsic surface, sustained release surface and lubrication surface are summarized. Furthermore,the research progress and prospects of various flexible anti-icing surfaces are emphatically described and the existing problems of these surfaces are particularly analyzed. The challenges and the prospective tendency of flexible anti-icing surfaces are also given according the current research.

Key words: flexible surface, anti-icing, lubrication, sustained release
Fig. 1 Preparation of organosilicon copolymers containing POSS structural units by different methods:(a) hydrosilylation,(b) RAFT,(c) click chemistry[27, 28]
Fig. 2 (a) Schematic illustration of anti-icing and deicing properties of a polyols-infused slippery surface.(b) Chemical strcture of amphiphilic copolymer P(PEGMA-co-GMA)[40]
Fig. 3 Method for preparing silicone sustained release flexible surface[41]
Fig. 4 (a) Schematic of the stimuli-responsive antifreeze secreting anti-icing coating;(b) schematic showing that the antifreeze liquid is secreted through the pores in response to contact with ice or frost forming on the surface, which results in melting of the ice or frost. Subsequently, the melt is removed via air motion or partially wicked back into the dermis[42]
Fig. 5 Schematic diagram of preparation of nanostructure PPy coating by electrodeposition[21]
Fig. 6 SEM images of lubricating oil before and after Rykalzewski freezing[54]
Fig. 7 Schematic diagram of the preparation of a earthworm-inspired polymer surface and its self-lubricating behavior[56,57,58]
Fig. 8 Preparation of poly(acrylic acid)(PAA) hydrophilic self-lubricating surface[62]
Fig. 9 Synthesis of the PAA-DA conjugate and schematic representation of the mussel-inspired construction of the anti-icing coating with an aqueous lubricating layer[63]
Fig. 10 Preparation of HBFP(Ⅲ)-PEG and LC-HBFP-PEG crosslinked networks[65,69,70]
Fig. 11 Synthesis of POSS-PDMAEMA-b-PSBMA and P(SBMA-co-FMA-co-AMA)[71, 72]
Fig. 12 Illustration of antifreeze protein from an insect(M. p. dzungarica) and selectively tethered MpdAFP on the PDA and GOPTS surfaces[75]
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