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Progress in Chemistry 2019, Vol. 31 Issue (5): 760-772 DOI: 10.7536/PC181004 Previous Articles   Next Articles

Application of Agroforestry Waste Biomass Adsorption Materials in Water Pollution Treatment

Jinxin Yi1,2, Zhipeng Huo1,**(), Abdullah M. Asiri3, Khalid A. Alamry3, Jiaxing Li1,3,**()   

  1. 1. Key Laboratory of Photovolatic and Energy Conservation Materials, Institute of Plasma Physics, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei 230031, China
    2. University of Science and Technology of China, Hefei 230026, China
    3. Chemistry Department, Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia
  • Received: Online: Published:
  • Contact: Zhipeng Huo, Jiaxing Li
  • About author:
    ** E-mail: (Zhipeng Huo);
    (Jiaxing Li)
  • Supported by:
    National High Technology Research and Development Program of China(21677146); National Natural Science Foundation of China(U1607102); Anhui Provincial Natural Science Foundation(1708085MB31)
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Environmental pollution has become one of the great challenges to the sustainable development of human society. Wastewater discharged from chemical, smelting and nuclear fuel cycle processes contain a lot of heavy metal ions, organic matter, and radionuclides. If discharged without treatment, it will bring great harm to the environment. The adsorption method for wastewater treatment has many advantages such as high efficiency, simple operation, no by-products, recyclability, and no secondary pollution, thus making it one of the significant methods for wastewater treatment. Due to the low cost, abundance in raw materials, and renewability of agroforestry waste biomass, the adsorption materials prepared on the basis of it are widely studied. In this paper, the research focuses on biochar, cellulose, and lignin, which are prepared from agroforestry waste biomass as raw materials, the preparation and modification methods of biochar, modification methods of natural cellulose, methods of modifying lignin, and their application in wastewater treatment are reviewed. The effects of adsorption properties on the adsorption of pollutants in water are discussed from the aspects of raw materials, preparation process, and modification methods. The problems of pollutant adsorption by biomass-based adsorption materials are pointed out and an outlook on their future research direction is made.

Key words: adsorption, agroforestry, biomass, biochar, cellulose, lignin, modification, water pollution
Fig. 1 Preparation and modification methods of agroforestry waste biomass based adsorbing materials
Table 1 Typical operating conditions for thermochemical processes and char production[33]
Process Temperature(℃) Residence time Char yield
Slow pyrolysis 400~600 min to days 20 wt%~40 wt%
Fast pyrolysis 400~600 ~1 s 10 wt%~20 wt%
Hydrothermal carbonization 180~300 1~12 h 30 wt%~60 wt%
Fig. 2 TGA of CDPC and CDPCO(A1); TOTH of CDPC and CDPCO(B1); BET specific surface areas of CDPC and CDPCO before and after MB adsorption(C1); size distributions of CDPC and CDPCO before and after MB adsorption(D1).Comparisons of(A2) the adsorption capacities toward organic pollutants of CDPC, CDPCO and cotton and the adsorption of MB on cotton(B2) and CDPCO(C2). C0=200 mg · L-1, m/V=0.1 g · L-1, T=298K[66]
Fig. 3 Modification methods for cellulose-based adsorbents and their usage in water treatment[96]
Fig. 4 Synthesis and metal ions adsorption scheme of SESD-PAA. Effect of(a) pH value(25 ℃, C0=150 mg · L-1, contact time=30 min),(b) initial concentration(25 ℃, pH=3.5 for Fe(Ⅲ) and 6 for other ions, contact time=30 min) and(c) contact time(25 ℃, C0=150 mg·L-1, pH=3.5 for Fe(Ⅲ) and 6 for other ions) on Zn(Ⅱ), Fe(Ⅲ), Cu(Ⅱ), and Cr(Ⅲ) ion adsorption[111]
Fig. 5 Schematic drawing of synthesis of cellulose-based bioadsorbents. Effects of(a) bioadsorbent dosage,(b) contact time,(c) solution pH, and(d) temperature on the dye removal efficiencies of AB93 and MB using the cellulose-based bioadsorbents[112]
Fig. 6 Modification methods for lignin-based adsorbents and their usage in water treatment[127]
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