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Progress in Chemistry 2019, Vol. 31 Issue (2/3): 337-350 DOI: 10.7536/PC180721 Previous Articles   Next Articles

Single-Ion Magnets Based on 3d Transition Metal

Lei Chen1,2,**(), Wen Zhao2, Gangji Yi2, Jianjun Zhou2, Aihua Yua2,**()   

  1. 1. School of Material Science and Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, China
    2. School of Environmental and Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, China
  • Received: Online: Published:
  • Contact: Lei Chen, Aihua Yua
  • About author:
    ** E-mail: (Lei Chen);
    (Aihua Yuan)
  • Supported by:
    National Natural Science Foundation(21601070); China Postdoctoral Science Foundation(2016M601751); Jiangsu Planned Projects for Postdoctoral Research Funds(1601037B)
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Single molecule magnets are potentially useful in quantum computing, high density data storage and molecular spintronics. 3d transition-metal-based single-ion magnets have attracted intensive interest because their structures are simple, and it is easy to explore the magneto-structural relationship, and achieve the higher barriers by tunable ligand field. Unifying the domestic and foreign research situation, the paper will show an overall perspective of the present single-ion magnets(SIMs) based on the 3d transition metal with the coordinated geometry, and highlight the relationship among the ligand field, the magnetic anisotropy and the behavior of single molecule magnet, which will provide a new route for the syntheses of single molecule magnets.

Key words: 3d transition metal, single-ion magnet, magnetic anisotropy, single molecule magnet
Fig. 1 Structure, d-orbital splitting, alternating-current magnetic susceptibility data and variable-field magnetization data for [FeI(C(SiMe3)3)2]-[14]
Fig. 2 Molecular structure of the mononuclear Fe(Ⅱ) and Co(Ⅱ) complexes[21]
Fig. 3 Structure(a) and variable-frequency out-of-phase ac susceptibility data(b) of the trigonal pyramidal complexes [(tpaMes)Fe]- [6]
Fig. 4 Structure, d-orbital energy level splitting and variable-frequency out-of-phase ac susceptibility data of the tetrahedral [Co(SPh)4]2-[29]
Fig. 5 Structure and variable-frequency out-of-phase ac susceptibility data for [{ArNdCMe}2(NPh)]Co(NCS)2(1) and [{ArNdCPh}2(NPh)]Co(NCS)2(2) [48]
Fig. 6 (a) two molecules showing short head-to-head contacts;(b) out-of-phase component[51]
Fig. 7 (a) The molecular structure of(HNEt3)+(CoⅡCo3ⅢL6)-;(b) The simplified d7 electron configuration;(c) The coordination model of the central Co(Ⅱ) ion;(d) variable-frequency out-of-phase ac susceptibility data; inset, Arrhenius analysis of the relaxation processes [68]
Fig. 8 ORTEP drawing of the anionic mononuclear manganese unit, variable-frequency out-of-phase ac susceptibility data, and field dependence of the normalized magnetization for(Ph4P)[Mn(opbaCl2)(py)2] [79]
Fig. 9 (a) Side view of molecular structure of the cation [Co(12-crown-4)2]2+;(b) Twist angle φ defined as the rotation angle of one coordination square away from the eclipse conformation to the other;(c) The angle α defined as the eight metal-ligand bonds make with the S8 axis passing through the metal atom Co;(d) Electronic configuration and d-orbital energy level diagram for the molecule from DFT calculation [90]
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