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Progress in Chemistry 2017, Vol. 29 Issue (9): 911-918 DOI: 10.7536/PC170510 Previous Articles   Next Articles

• Review •

Photocatalytic Reductive Debromination of Polybrominated Diphenyl Ethers

Yukun Zhao, Yuanyuan Wang, Hongwei Ji, Wanhong Ma, Chuncheng Chen*, Jincai Zhao*   

  1. Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
  • Received: Revised: Online: Published:
  • Supported by:
    The work was supported by the National Basic Research Program of China (973 Program)(No.2013CB632405),NSFC (No.21590811,21521062,21525729),and the CAS Interdisciplinary Innovation Team of the Chinese Academy of Sciences.
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Global extensive concerns have been caused by polybrominated diphenyl ethers (PBDEs),because of their universal existence and potential toxicity in ecological environment. The use of solar energy, high selectivity and the mild reaction conditions make photocatalysis become a promising technique for the removal of these pollutants. Recently, great progress has been made in photocatalytic degradation of polyhalogenated organic pollutions. This review mainly focuses on TiO2-based photocatalytic reduction of PBDEs, which are typical polyhalogenated aromatic hydrocarbons. The ways to improve photocatalytic reductive efficiency and the reaction mechanism have been described. In addition, the promising future of PBDEs photocatalytic reductive debromination is prospected.
Contents
1 Introduction
2 An overview of PBDEs
3 Photocatalytic reductive debromination of PBDEs
3.1 Photocatalytic reductive debromination based on TiO2
3.2 Photoreductive debromination based on halogen bonding under visible light
4 Proton-coupled electron transfer based on photocatalytic reductive process of PBDEs
5 Conclusion
Key words: polybrominated diphenyl ethers, photocatalytic, reductive debromination, TiO2

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