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Progress in Chemistry 2015, Vol. 27 Issue (6): 763-774 DOI: 10.7536/PC150228 Previous Articles   Next Articles

• Review and evaluation •

Self-Assembly of Mechanically Interlocked Structures via Metal-Mediated Coordination Cooperating with Host-Guest Recognition

Ye Yang, Lin Zheping, Jin Wenlu, Wang Shuping, Wu Jing, Li Shijun*   

  1. College of Material, Chemistry and Chemical Engineering, Hangzhou Normal University, Hangzhou 310036, China
  • Received: Revised: Online: Published:
  • Contact: 10.7536/PC150228 E-mail:l_shijun@hznu.edu.cn
  • Supported by:
    The work is supported by the National Natural Science Foundation of China (No. 21072039, 21172049, 91127010), the Program for Changjiang Scholars and Innovative Research Team in Chinese University (IRT 1231), and the Zhejiang Provincial Natural Science Foundation of China (No. LZ13B030001).
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Mechanically interlocked structures are a kind of supramolecular entities with unique properties. They have attracted much attention not only because of their fascinating aspect of topologies, but also due to their great potential applications in nanotechnology, biology, and material science, as well as important bases for the preparation of molecular machines. This article summarizes new progress in the preparation of rotaxanes, catenanes, and other mechanically interlocked structures assembled via coordination interactions, especially focuses on the examples using metal-mediated coordination interactions as building ways cooperating with host-guest chemistry. Because coordination bonds are easy bonding, dynamically reversible, and easily controllable, the usage of metal-mediated coordination for constructing mechanically interlocked structures can greatly improve the preparation efficiency, and benefit to realizing the reversible regulation of mechanically interlocked structures.

Contents
1 Introduction
2 Self-assembly of rotaxanes via metal-mediated coordination
3 Self-assembly of catenanes via metal-mediated coordination
4 Self-assembly of other mechanically interlocked structures via metal-mediated coordination
5 Conclusion

Key words: host-guest chemistry, coordination, self-assembly, rotaxanes, catenanes, mechanically interlocked structures

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