English
新闻公告
More
化学进展 2009, Vol. 21 Issue (10): 2100-2114 前一篇   后一篇

• 综述与评论 •

烧绿石型复合氧化物的结构、制备及其光催化性能

唐新德*;叶红齐;马晨霞;刘辉   

  1. (中南大学化学化工学院 长沙 410083)
  • 收稿日期:2008-10-29 修回日期:2008-12-06 出版日期:2009-10-24 发布日期:2009-10-09
  • 通讯作者: 唐新德 E-mail:txd759@sina.com
  • 基金资助:

Structure and Preparation of Pyrochlore-Type Complex Oxides and Their Photocatalytic Performance

Tang Xinde*;  Ye Hongqi;  Ma Chenxia;  Liu Hui   

  1. (College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China )
  • Received:2008-10-29 Revised:2008-12-06 Online:2009-10-24 Published:2009-10-09
  • Contact: Tang Xinde E-mail:txd759@sina.com

本文系统介绍了烧绿石型复合氧化物的结构特点;综述了近年来国内外烧绿石型复合氧化物的制备方法及其影响因素;总结了这类材料在光催化降解有机物和光催化分解水方面的研究进展,探讨了光催化反应机理及影响光催化活性的因素;分析了烧绿石型复合氧化物的应用前景,并展望了今后研究的发展方向。

The structure properties of pyrochlore-type complex oxides are introduced systematically, whose preparation methods and influence factors in recent years are also summarized. The progress of these materials in photocatalytically degrading organic compounds and splitting water is reviewed,and the photocatalytic mechanism and factors influencing photocatalytic performance are discussed. The potential applications of pyrochlore-type oxides are analyzed, in addition, the ideas for further research are presented.

Contents
1 Introduction
2 Structures of pyrochlore-type complex oxides
3 Preparation methods of pyrochlore-type complex oxides
3.1 The gas-state reaction method
3.2 The solid-state reaction method
3.3 The liquid-state reaction method
4 Photocatalytic performance of pyrochlore-type complex oxides
4.1 Photodegradation of organic compounds
4.2 Photocatalytic water splitting
5 Conclusions and prospect

中图分类号: 

()

[ 1 ]  干福熹(Gan F X) . 信息材料( Information Materials) . 天津: 天津大学出版社(Tianjing: Tianjing university press) , 2000. 203 —224
[ 2 ]  Shimakawa Y, Kubo Y, Hamada N , et al . Physical Review B ,1999 , 59 : 1249 —1254
[ 3 ]  Takeda T, Kanno R , Yamamoto Y, et al . Journal of Materials Chemistry , 1999 , 9 : 215 —222
[ 4 ]  Khasanov R , Eshchenko G D , Karpinski J , et al . Physical Review Letters , 2004 , 93 : 1570041-1570044
[ 5 ]  Colomban P. Annales de Chimie Science des Materiaux , 1999 , 24 :1 —8
[ 6 ]  Kramer S A , Tuller H L. Solid State Ionics , 1995 , 82 : 15 —23
[ 7 ]  Porat O , Spears MA , Heremans C , et al . Solid State Ionics , 1996 ,86P88 : 285 —288
[ 8 ]  Holtappels P , Poulsen F W, Mogensen M. Solid State Ionics , 2000 ,135 : 675 —679
[ 9 ]  Shimura T, Komori M, Iwahara H. Solid State Ionics , 1996 , 86P88 :685 —689
[10 ]  Mori M, Tompsett G M, Sammes N M, et al . Solid State Ionics ,2003 , 158 : 79 —90
[11 ]  Zhuiykov S. International Journal of Hydrogen Energy , 1996 , 21(9) : 749 —759
[12 ]  Labrincha J A , Frade J R , Marques F B. Solid State Ionics , 1997 ,99 : 33 —40
[13 ]  Wuensch B J , Eberman K W, Heremans C , et al . Solid State Ionics , 2000 , 129 (1/4) : 111 —133
[14 ]  Bondah-Jagalu V , Bramwell S T. Cannadian Journal of Physics ,2001 , 79 (11/12) : 1381 —1385
[15 ]  Matsuhira K, Hinatsu Y, Tenya K, et al . Journal of the Physical Society of Japan , 2002 , 71 (6) : 1576 —1582
[16 ]  Fujinaka H , Kinamura N , Koizumi M, et al . Materials Research Bulletin , 1979 , 14 (9) : 1133 —1137
[17 ]  Troyanchuk I O , Derachenko V N. Sov. Phys. Solid State , 1988 ,30 : 2003 —2008
[18 ]  Subramanian MA , Torardi C C , Johnson D C , et al . Journal of Solid State Chemistry , 1988 , 72 : 24 —30
[19 ]  Reimers J N , Greedan J E , Kremer R K, et al . Physical Review B ,1991 , 43 : 3387 —3392
[20 ]  Raju N P , Greedan J E , Subramanian M A. Physical Review B ,1994 , 49 : 1086 —1091
[21 ]  Shimakawa Y, Kubo Y, Manako T. Nature , 1996 , 379 : 53 —57
[22 ]  Teraoka Y, Torigoshi K, Yamaguchi H , et al . Journal of Molecular Catalysis A-Chemical , 2000 , 155 (1P2) : 73 —80
[23 ]  Park S , Hwang H J , Moon J . Catalysis Letters , 2003 , 87 (3/4) :219 —223
[24 ]  Zahir M H , Matsuda K, Katayama S , et al . Journal of Ceramic Society of Japan , 2002 , 110 (11) : 963 —969
[25 ]  Chakoumakos B C. Journal of Solid State Chemistry , 1984 , 53 : 120
[26 ]  Subramanian M A , Aravamudan G, Rao G V S , et al . Journal of Solid State Chemistry , 1983 , 15 : 55
[27 ]  Ismunandar D , Kennedy B J , Hunter B A. Journal of Alloysand Compounds , 2000 , 302 : 94 —100
[28 ]  Greedan J E. Journal of Alloys and Compounds , 2006 , 408/412 :444 —455
[29 ]  Brendan J K. Physica , 1998 , 241/243 : 303 —310
[30 ]  Isasi J , Lpez M L , Veiga M L , et al . Journal of Solid State Chemistry , 1995 , 116 : 290 —295
[31 ]  Erickson E E , Gray D , Taylor K, et al . Materials Research Bulletin , 2002 , 37 : 2077 —2083
[32 ]  Helean KB , Ushakov S V , Brown C E , et al . Journal of Solid State Chemistry , 2004 , 177 : 1858 —1866
[33 ]  Isasi J , Lpez ML , Veiga ML , et al . Solid State Ionics , 1996 , 89 :321 —326
[34 ]  Wilde P J , Catlow C R A. Solid State Ionics , 1998 , 112 : 173 —183
[35 ]  Lian J , Weber W J , Jiang W, et al . Nuclear Instruments and Methods in Physics Research B , 2006 , 250 : 128 —136
[36 ]  Kahlenberg V , Bhm H. Journal of Alloy and Compounds , 1995 ,223 : 142 —146
[37 ]  Uma S , Kodialam S , Yokochi A , et al . Journal of Solid State Chemistry , 2000 , 155 : 225 —228
[38 ]  Heremans C , Wuensch B J . Journal of Solid State Chemistry , 1995 ,117 : 108 —121
[39 ]  Tabira Y, Withers R , Thompson J , et al . Journal of Solid State Chemistry , 1999 , 142 : 393 —399
[40 ]  Haynes D J , Berry D A , Shekhawat D , et al . Catalysis Today ,2008 , 136 (3P4) : 206 —213
[41 ]  Beck N K, Steiger B , Scherer G G, et al . Full Cells , 2006 , 6 (1) :26 —30
[42 ]  Gao F , Liu Y F , Liu X Q. Sensors and Actuators B : Chemical ,2001 , 77 (3) : 653 —656
[43 ]  Saruhan B , Francois P , Fritscher K, et al . Surface and Coatings Technology , 2004 , (182) : 175 —183
[44 ]  Suzuki M, Watanabe T, Takenaka T, et al . Journal of the European Ceramic Society , 2006 , (26) : 2155 —2159
[45 ]  Cupta H C , Brown S , Rani N , et al . International Journal of Inorganic Materials , 2001 , 3 : 983 —986
[46 ]  Zou Z G, Ye J H , Arakawa H. Solid State Communications , 2000 ,(116) : 259 —263
[47 ]  Zou Z G, Ye J H , Arakawa H. Materials Science and Engineering B , 2001 , 79 : 83 —85
[48 ]  Zou Z G, Ye J H , Arakawa H. Joural of Materials Research , 2001 ,(16) : 35 —37
[49 ]  Zou Z G, Ye J H , Arakawa H. The Journal of Physical Chemistry ,2002 , 106 : 517 —520
[50 ]  Yamamura H , Nishino H , Kakinuma K. Journal of Physics and Chemistry of Solids , 2007 , 1 : 1 —7
[51 ]  Tong Y P , Zhu J W, Lu L D , et al . Journal of Alloys and Compounds , 2008 , 465 : 280 —284
[52 ]  谢亚红(Xie YH) , 刘瑞泉(Liu R Q) , 李志杰(Wang ZJ ) 等. 无机化学学报(Chinese Journal of Inorganic Chemistry) , 2004 , 20(5) : 551 —554.
[53 ]  Bansal N P , Zhu D M. Materials Science and Engineering : A ,2007 , 45 (1P2) : 192 —195
[54 ]  Wang J D , Xie YH , Zhang Z F , et al . Materials Research Bulletin ,2005 , 40 (8) : 1294 —1302
[55 ]  Fjeld H , Haugsrud R , Gunn·s A E , et al . Solid State Ionics , 2008 ,179 : 1849 —1853
[56 ]  Xie Y H , Wang J D , Liu R Q , et al . Solid State Ionics , 2004 , 168(1/2) : 117 —121
[57 ]  Rao K K, Anantharamulu N , Salagram M, et al . Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy , 2007 , 66(3) : 646 —649
[58 ]  Zanetti S M, Pereira M G S , Nono M C A. Journal of the European Ceramic Society , 2007 , 27 (13P15) : 3647 —3650
[59 ]  Rao K K, Banu T, Vithal M, et al . Materials Letters , 2002 , 54 :(2/3) , 205 —210
[60 ]  Kahoul A , Nkeng P , Hammouche A , et al . Journal of Solid State Chemistry , 2001 , 161 (2) : 379 —384
[61 ]  Tong Y P , Wang Y P , Yu Z X, et al . Materials Letters , 2008 , 62 :889 —891
[62 ]  Tong Y P , Lu L D , Yang X J , et al . Solid State Sciences , 2008 ,10 : 1 —5
[63 ]  Yang X N , Huang B B , Wang H B , et al . Journal of Crystal Growth , 2004 , 270 (1P2) : 98 —101
[64 ]  Zhang H P , LüM K, Liu SW, et al . Thin Solid Films , 2008 , 517 :764 —768
[65 ]  Hector A L , Wiggin S B. Journal of Solid State Chemistry , 2004 ,177 : 139 —145
[66 ]  Cheng J , Wang H L , Hao Z P , et al . Catalysis Communications ,2008 , 9 : 690 —695
[67 ]  刘亚飞(Liu Y H) , 刘杏芹(Liu S Q) . 无机化学学报(Chinese Journal of Inorganic Chemistry) , 1999 , 15 (3) : 293 —300
[68 ]  Zhao H , Feng S H , Xu W, et al . Journal of Material Chemistry ,2000 , 10 (2) : 479 —482
[69 ]  Li K W, Wang H , Yan H. Journal of Molecular Catalysis A:Chemical , 2006 , 249 : 65 —70
[70 ]  Li K W, Zhang T T, Wang H , et al . Journal of Solid State Chemistry , 2006 , 179 (4) : 1029 —1034
[71 ]  Chen D , Xu R. Materials Research Bulletin , 1998 , 33 (3) : 409 —417
[72 ]  Mao Y C Li G S , Sun Y Y, et al . Journal of Solid State Chemistry ,2000 , 149 (2) : 314 —319
[73 ]  张进治(Zhang J Z) , 张婷婷(Zhang T T) , 汪浩(Wang H) 等. 功能材料(Chinese Journal of funcional material) , 2008 , 39 : 721 —723
[74 ]  Zeng J , Wang H , Zhang YC , et al . Journal of Physcial Chemstry C ,2007 , 111 : 11879 —11887
[75 ]  Fujishima A , Honda K. Nature , 1972 , 238 (53P58) : 37
[76 ]  刘守新(Liu S X) , 刘鸿(Liu H) . 光催化及光电催化基础与应用(Basics and Applications of Photocatalysis and Photoelectricity-Catalysis) . 北京: 化学工业出版社(Beijing : Chemical Industry Press) , 2006 , 206 —207
[77 ]  Garza-Tovar L L , Torres-Martínez L M, Rodríguez D B , et al .Journal of Molecular Catalysis A: Chemical , 2006 , 247 : 283 —290
[78 ]  Tong Y P , Xue P P , Lu L D , et al . Materials Science and Engineering B , 2008 , 150 : 194 —198
[79 ]  Zhang L L , Zhong H , Zhang W G, et al . Journal of Alloys and Compounds , 2008 , 463 : 466 —470
[80 ]  Luan J F , Zou Z G, Lu M H , et al . Journal of Crystal Growth ,2004 , 273 : 241 —247
[81 ]  Luan J F , Hao X P , Zheng S R , Luan GY, et al . Journal of Materials Science , 2006 , 41 : 8001 —8012
[82 ]  Luan J F , Zou Z G, Lu M H , et al . Research on Chemical Intermediate , 2006 , 32 : 31 —42
[83 ]  Luan J F , Zheng S R , Hao X P , et al . Journal of the Brazilan Chemical Society , 2006 , 17 : 1368 —1376
[84 ]  Luan J F , Lu M H , Zheng S R , et al . Journal of Materials Science ,2005 , 40 : 4905 —4909
[85 ]  Xiao Q , Zhou Q T, Zhang J , et al . Journal of Alloys and Compounds , 2009 , 468 : L9 —L12
[86 ]  Yao W F , Wang H , Xu X H , et al . Applied Catalysis A: General ,2004 , 259 : 29 —33
[87 ]  Zou Z G, Ye J H , Arakawa H , et al . Journal of Molecular Catalysis A: Chemical , 2002 , 168 : 289 —297
[88 ]  Zou Z G, Ye J H , Arakawa H. Chemistry of Materials , 2001 , 13 :1765 —1769
[89 ]  Zou Z G, Ye J H , Arakawa H. Chemical Physics Letters , 2001 ,333 : 57 —62
[90 ]  Zou Z G, Ye J H , Arakawa H. International Journal of Hydrogen Energy , 2003 , 28 : 663 —669
[91 ]  Zou Z G, Ye J H , Arakawa H. Topics in Catalysis , 2003 , 22 :107 —110
[92 ]  Wang J H , Zou Z G, Ye J H. Journal of Alloys and Compounds ,2004 , 377 : 248 —252
[93 ]  Wang J H , Zou Z G, Ye J H. Journal of Physics and Chemistry of Solids. 2005 , 66 : 349 —355
[94 ]  Wang J H , Zou Z G, Ye J H. Materical Science , 2003 , 423 (4) :485 —490
[95 ]  Sato S , White J M. Chemical Physics Letters , 1980 , 72 : 83
[96 ]  Hara M, Nunoshige J , Takata T, et al . Chemical Communications ,2003 , 24 : 3000 —3001
[97 ]  Kato H , Asakura K, Kudo A. Journal of the American Chemical Society , 2003 , 125 : 3082 —3089
[98 ]  Domen K, Naito S , Onishi T, et al . Journal of Physical Chemistry ,1982 , 86 : 3657 —3661
[99 ]  Domen K, Kudo A , Onishi T. Journal of Physical Chemistry , 1986 ,90 : 292 —295
[100 ] Sohn J M, Woo S I. Applied Catalysis A: General , 2003 , 249 :375 —384
[101 ] Kim H G, Hwang D W, Kim J , et al . Chemical Communications ,1999 , 1077 —1078
[102 ] Sakata T, Hashimoto K, Kawait T. Journal of Physical Chemistry ,1984 , 88 : 5214 —5221
[103 ] Li Z, Xu N , Chen Y, et al . Research on Chemical intermediate ,2005 , 31 (4P6) : 529 —534
[104 ] Li Y X, Chen G, Zhang H J , et al . Materials Research Bulletin ,2009 , 44 (4) : 741 —746
[105 ] Maruyama Y, Irie H , Hashimoto K. Journal of Physical Chemistry B ,2006 , 110 : 23274 —23278
[106 ] Ikeda S , Fubuki M, Takahara Y K, et al . Applied CatalysisA:General , 2006 , 300 : 186 —190
[107 ] Abe R , Higashi M, Zou Z G, et al . Chemisty Letters , 2004 , 33 :954 —955
[108 ] Abe R , Higashi M, Sayama K, et al . Journal of Physical Chemistry B , 2006 , 110 : 2219 —2226
[109 ] Higashi M, Abe R , Sayama K, et al . Chemistry Letters , 2005 , 34 :122 —1123
[110 ] Uno M, Kosuga A , Okui M, et al . Journal of Alloys and Compounds , 2006 , 420 : 291 —297
[111 ] Uno M, Kosuga A , Okui M, et al . Journal of Alloys and Compounds , 2005 , 400 : 270 —275
[112 ] Pavlov R S , Castello J B C , Marza V B , et al . Journal of the American Ceramic Society , 2002 , 85 (5) : 1197 —1202
[113 ] Srivastava A M. Materials Research Bulletin , 2002 , 37 (4) : 745 —751
[114 ] 李凤生(Li F S) . 超细粉体技术( Technology of Superfine Powder) . 北京: 国防工业出版社(Beijing: National Defence Industry Press) , 2000 , 3 —4
[115 ] Machida M, Yabunaka J , Kijima T. Chemistry of Materials , 2000 ,12 : 812 —817
[116 ] Machida M, Murakami S , Kijima T. Journal of Physical Chemistry B , 2001 , 105 : 3289 —3294
[117 ] Machida M, Yabunaka J , Kijima T, et al . International Journal of Inorganic Materials , 2001 , 3 : 545 —550
[118 ] Kudo A , Omori K, Kato H. Journal of the American Chemical Society , 1999 , 121 : 11459 —11467
[119 ] Hosogi Y, Tanabe K, Kato H , et al . Chemistry of Materials , 2008 ,20 : 1299 —1307
[120 ] Hosogi Y, Tanabe K, Kato H , et al . Chemistry Letters , 2004 , 33 :28 —29
[121 ] Bak T, Nowotny J , Rekas M, et al . International Journal of Hydrogen Energy , 2002 , 27 : 991 —1022

[1] 王丹丹, 蔺兆鑫, 谷慧杰, 李云辉, 李洪吉, 邵晶. 钼酸铋在光催化技术中的改性与应用[J]. 化学进展, 2023, 35(4): 606-619.
[2] 刘雨菲, 张蜜, 路猛, 兰亚乾. 共价有机框架材料在光催化CO2还原中的应用[J]. 化学进展, 2023, 35(3): 349-359.
[3] 李锋, 何清运, 李方, 唐小龙, 余长林. 光催化产过氧化氢材料[J]. 化学进展, 2023, 35(2): 330-349.
[4] 范倩倩, 温璐, 马建中. 无铅卤系钙钛矿纳米晶:新一代光催化材料[J]. 化学进展, 2022, 34(8): 1809-1814.
[5] 马晓清. 石墨炔在光催化及光电催化中的应用[J]. 化学进展, 2022, 34(5): 1042-1060.
[6] 李晓微, 张雷, 邢其鑫, 昝金宇, 周晋, 禚淑萍. 磁性NiFe2O4基复合材料的构筑及光催化应用[J]. 化学进展, 2022, 34(4): 950-962.
[7] 庞欣, 薛世翔, 周彤, 袁蝴蝶, 刘冲, 雷琬莹. 二维黑磷基纳米材料在光催化中的应用[J]. 化学进展, 2022, 34(3): 630-642.
[8] 占兴, 熊巍, 梁国熙. 从废水到新能源:光催化燃料电池的优化与应用[J]. 化学进展, 2022, 34(11): 2503-2516.
[9] 王文婧, 曾滴, 王举雪, 张瑜, 张玲, 王文中. 铋基金属有机框架的合成与应用[J]. 化学进展, 2022, 34(11): 2405-2416.
[10] 唐晨柳, 邹云杰, 徐明楷, 凌岚. 金属铁络合物光催化二氧化碳还原[J]. 化学进展, 2022, 34(1): 142-154.
[11] 葛明, 胡征, 贺全宝. 基于尖晶石型铁氧体的高级氧化技术在有机废水处理中的应用[J]. 化学进展, 2021, 33(9): 1648-1664.
[12] 赵依凡, 毛琦云, 翟晓雅, 张国英. 钼酸铋光催化剂的结构缺陷调控[J]. 化学进展, 2021, 33(8): 1331-1343.
[13] 陈肖萍, 陈巧珊, 毕进红. 光催化降解土壤中多环芳烃[J]. 化学进展, 2021, 33(8): 1323-1330.
[14] 郭俊兰, 梁英华, 王欢, 刘利, 崔文权. 光催化制氢的助催化剂[J]. 化学进展, 2021, 33(7): 1100-1114.
[15] 毕洪飞, 刘劲松, 吴正颖, 索赫, 吕学良, 付云龙. 硫化铟锌的改性合成及光催化特性[J]. 化学进展, 2021, 33(12): 2334-2347.