收稿日期: 2024-06-21
修回日期: 2024-10-10
网络出版日期: 2025-03-19
基金资助
中组部“千人计划”青年项目(40127002)
Post-combustion CO2 Capture Materials
† These authors contributed equally to this work.
Received date: 2024-06-21
Revised date: 2024-10-10
Online published: 2025-03-19
Supported by
the Youth Funding Project of the "Thousand Talents Program" of the Organization Department of the Central Committee of the Communist Party of China(40127002)
工业的持续发展带来了巨大的经济效益,但也对环境造成了极大的危害。化石能源燃烧排放的超多CO2被排放到自然环境中,对环境和人类健康构成威胁。所以人们正在努力开发能够有效捕获CO2的材料。目前CO2捕获主要发生在化石燃料燃烧后,依据CO2吸附剂设计标准,多种多样的CO2捕获材料被设计开发出来,有固体吸附剂、液体吸附剂和多相吸附剂。各种吸附剂的吸附机理也不尽相同,包括吸附、吸收或两种机理共同作用。本综述聚焦于目前常见的各类吸附剂的捕获性能、吸收机理和优缺点,分别对胺溶液吸收剂、沸石基吸附剂、离子液体类吸附剂、碳基吸附剂、金属有机框架材料、共价有机框架材料、金属氧化物材料和生物聚合物纳米复合材料进行介绍,并对各类CO2吸附材料未来的发展做出展望。
江佳佳 , 赵俊虎 , 喻勤 , 张甜 . 燃烧后CO2捕获材料[J]. 化学进展, 2025 , 0(0) . DOI: 10.7536/PC240608
The sustained development of industry has brought enormous economic benefits, but it has also caused great harm to the environment. The excessive CO2 emissions from fossil fuel combustion are released into the natural environment, posing a threat to the environment and human health. So people are working hard to develop materials that can effectively capture CO2. At present, CO2 capture mainly occurs after the combustion of fossil fuels. According to the design standards for CO2 adsorbents, a variety of CO2 capture materials have been designed and developed, including solid adsorbents, liquid adsorbents, and multiphase adsorbents. The adsorption mechanisms of various adsorbents are also different, including adsorption, absorption, or a combination of both mechanisms.This review focuses on the capture performance, absorption mechanism, advantages and disadvantages of various common types of current adsorbents, and introduces amine solution absorbents, zeolite-based adsorbents, ionic liquids-based adsorbents, carbon-based adsorbents, metal-organic framework materials, covalent organic framework materials, metal-oxide materials, and biopolymer nanocomposites, respectively, with an outlook of the future development of CO2 adsorbent materials.
Contents
1 Introduction
1.1 Current status and hazards of CO2 emissions
1.2 CO2 capture technology
1.3 Criteria for designing CO2 capture materials
2 CO2 capture materials
2.1 Amine solution absorbents
2.2 Zeolites based adsorbents
2.3 Ionic liquids absorbents(ILs)
2.4 Carbon-based adsorbents
2.5 Metal organic framworks(MOF)
2.6 Covalent organic frameworks(COF)
2.7 Metal oxide sorbents
2.8 Biopolymeric nanocomposites
3 Comparison and Prospect of Capture Materials
4 Conclusion
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