• 综述 •
宋欢, 邹琦, 陆克定. HO2非均相摄取系数的测量与参数化[J]. 化学进展, 2021, 33(7): 1175-1187.
Huan Song, Qi Zou, Keding Lu. Parameterization and Application of Hydroperoxyl Radicals(HO2) Heterogeneous Uptake Coefficient[J]. Progress in Chemistry, 2021, 33(7): 1175-1187.
HO2自由基与环境大气气溶胶的非均相反应是HO2自由基的重要汇之一,对大气氧化能力有重要影响,对大气颗粒物的物化性质等进一步产生影响。HO2的非均相反应过程的定量描述对不同地区大气氧化性与臭氧生成能力等问题的探求具有重要意义。目前不同研究小组测量的摄取系数可相差3到5个数量级,深入探究不同条件下不同种类气溶胶对HO2自由基的非均相摄取机制,对摄取机制进行参数化表达,并准确测量摄取系数是量化其环境影响的关键。本文深入介绍了HO2非均相摄取的原理与参数化表达,总结了已有的研究结果与进展,对不同的影响因素进行总结分析,并对此领域未来的发展方向提出建议与展望。
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