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化学进展 2012, Vol. 24 Issue (05): 659-673   后一篇

• 综述与评论 •

离子液体表/界面性质与结构

闫燕, 杨启炜, 邢华斌*, 苏宝根, 任其龙   

  1. 浙江大学生物质化工教育部重点实验室 化学工程与生物工程学系 杭州 310027
  • 收稿日期:2011-09-01 修回日期:2011-12-01 出版日期:2012-05-24 发布日期:2012-04-10
  • 基金资助:
    国家自然科学基金项目(No.20936005,21006082)和国家高技术发展计划(863)项目(No.2012AA040211)资助
下载PDF ( 1443 ) 引用
导出 被引次数 ( 17 | 3 )

Surface/Interfacial Properties and Structures of Ionic Liquids

Yan Yan, Yang Qiwei, Xing Huabin, Su Baogen, Ren Qilong   

  1. Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Department of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China
  • Received:2011-09-01 Revised:2011-12-01 Online:2012-05-24 Published:2012-04-10
离子液体与气体、溶剂等物质组成的多相体系为吸收、萃取、两相催化等技术的发展提供了新的平台。离子液体的表/界面性质与结构是含离子液体多相体系的重要科学问题,可在介观尺度下显著影响多相体系反应和分离过程的效率。近年来,离子液体表/界面性质和结构的研究得到了广泛的关注。本文综述了离子液体及其与水、有机溶剂组成的混合物的表/界面张力及结构研究进展,介绍了现有的研究方法、研究对象与研究成果,归纳了离子液体及其混合物表/界面张力及结构的变化规律,分析了表/界面结构与表/界面张力之间的关系,探讨了离子液体表/界面研究存在的问题和未来的发展方向。
关键词： 离子液体, 表/界面性质, 表/界面结构, 分子模拟, 非线性光谱
Heterogeneous systems containing ionic liquids (ILs) with gases and solvents extend the acpplications of ILs in absorption, extraction and heterogeneous catalysis. In recent years, the surface/interfacial properties and surface/interfacial structures of ionic liquids have been widely studied, because they are important due to their remarkable effects on heterogeneous reactions and separation efficiency. In this article, the surface/interfacial tension,as well as the surface/interfacial structures of ILs and their mixtures with water and organic solvents are summarized. The research methods, objectives and results are introduced. The relationship between surface/interfacial tension and surface/interfacial structures is elucidated. Finally, the exiting problems and development prospects of the studies on surface/interfacial properties and surface/interfacial structures of ILs are discussed.

Contents
1 Introduction
2 Surface tension of ionic liquids and their mixtures
2.1 Surface tension of ionic liquids
2.2 Surface tension of ionic liquid mixtures
3 Liquid/liquid interfacial tension of ionic liquids
4 Surface/interfacial structures of ionic liquids
4.1 Direct recoil spectroscopy
4.2 Neutron and X-ray reflectivity
4.3 Ultra-high vacuum systems
4.4 Non-linear spectroscopy
4.5 Molecular dynamic simulation
5 Conclusion and outlook

Key words: ionic liquids, surface/interfacial properties, surface/interfacial structures, molecular dynamic simulation, non-linear spectroscopy

中图分类号: 

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摘要

离子液体表/界面性质与结构