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化学进展 2011, Vol. 23 Issue (8): 1782-1794 前一篇   

• 综述与评论 •

藻类去除水体中重金属的机理及应用

支田田1, 程丽华2*, 徐新华2, 张林1, 陈欢林1   

  1. 1. 浙江大学化学工程与生物工程学系 杭州 310027;
    2. 浙江大学环境工程系 杭州 310058
  • 收稿日期:2010-10-01 修回日期:2010-12-01 出版日期:2011-08-24 发布日期:2011-07-25
  • 通讯作者: 程丽华 E-mail:chenglihua@zju.edu.cn
  • 基金资助:

    国家自然科学基金项目(No. 21076177)、教育部博士点基金项目(No. 200803350077)、中央高校基本科研业务费专项资金项目(No.2009QNA6007, KYJD09011)和浙江省自然科学基金项目(No.Y4100222)资助

Advances on Heavy Metals Removal from Aqueous Solution by Algae

Zhi Tiantian1, Cheng Lihua2*, Xu Xinhua2, Zhang Lin1, Chen Huanlin1   

  1. 1. Department of Chemical and Biochemical Engineering, Zhejiang University, Hangzhou 310027, China;
    2. Department of Environmental Engineering, Zhejiang University, Hangzhou 310058, China
  • Received:2010-10-01 Revised:2010-12-01 Online:2011-08-24 Published:2011-07-25

重金属污染水体的修复,以及含重金属工业废水的处理关乎地球上生物的健康发展。利用低耗能、高修复效率、环境友好、适用范围广泛的藻类去除水体中的重金属,已越来越受到研究者的关注。本文综述了国内外藻类去除水体中重金属的研究进展。分析了藻类去除重金属的生化结构;重点阐述了藻类吸附及富集重金属的机理;讨论了活藻体和死亡藻体用于水体中重金属去除的应用及影响因素,并比较了两者的适用范围及筛选标准;最后指出此领域尚存在的问题,展望了藻类去除重金属的未来发展方向。

Environmental contamination by toxic heavy metals is a significant global issue. Heavy metals removal from aqueous solution by algae, due to its good performance, low cost, environmental friendliness and wide applicability, have received increasing attention in recent years. In this work, the advances on algal heavy metals removal from aqueous solution are reviewed. The properties of algal cell wall constituents and their key functional groups are analyzed. The mechanisms of algal bioadsorption and bioaccumulation are then elaborated. Afterwards, the application of living and nonliving algae in heavy metal removal including their removal capacity and the effects of adsorption conditions are compared, and the selection criteria of algae are introduced. Finally, the existing deficiencies and suggestions on further study of the proposed algal bioremoval technology are discussed.

Contents
1 Introduction
2 Algal cell wall constitution and their key functional groups for heavy metal removal
3 Mechanisms for algal bioremoval of heavy metals
3.1 Bioadsorption
3.2 Bioaccumulation
4 Application of living and nonliving algaes in heavy metal bioremoval
4.1 Usage of living algae
4.2 Usage of nonliving algae
4.3 Comparison of living and nonliving algae
5 Outlook

中图分类号: 

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[1] 胡国飞(Hu G F), 孟祥和(Meng X H). 重金属废水处理(Heavy Mental Wastewater Treatment). 北京: 化学工业出版社(Beijing: Chemistry Industry Press), 2000. 17-51
[2] 赵由才(Zhao Y C). 危险废物处理技术(Hazard waste treatment technology). 北京: 化学工业出版社(Beijing: Chemistry Industry Press), 2003. 243-244
[3] Gupta V K, Rastogi A. J. Hazard. Mater., 2008, 152(1): 407-414
[4] Jacinto M, David C, Perez T R, De Jesus B R. Ecol. Eng., 2009, 35(5): 856-860
[5] Debelius B, Forja J M, Delvalls A, Lubian L M. Ecotox. Environ. Safe., 2009, 72(5): 1503-1513
[6] Deng L P, Zhang Y, Qin J, Wang X T, Zhu X B. Miner. Eng., 2009, 22(4): 372-377
[7] Vilar V, Botelho C, Pinheiro J, Domingos R F, Boaventure R. J. Hazard. Mater., 2009, 163(2/3): 1113-1122
[8] Volesky B. Hydrometallurgy, 2001, 59(2/3): 203-216
[9] Wilke A, Buchholz R, Bunke G. Environ. Biotechnol., 2006, 2(2): 47-56
[10] Wang J L, Chen C. Biotechnol. Adv., 2009, 27(2): 195-226
[11] Deng L, Zhu X, Wang X, Su Y, Su H. Biodegradation, 2007, 18(4): 393-402
[12] 潘进芬(Pan J F).中科院海洋研究所硕士论文(Master's Dissertation of Institute of Oceanology,Chinese Academy of Science),2000
[13] Liu Y H, Cao Q L, Luo F, Chen J. J. Hazard. Mater., 2009, 163(2/3): 931-938
[14] Chen J Z, Tao X C, Xu J, Zhang T, Liu Z L. Process Biochem., 2005, 40(12): 3675-3679
[15] Gong R M, Ding Y, Liu H J, Chen Q Y, Liu Z L. Chemosphere, 2005, 58(1): 125-130
[16] 王建龙(Wang J L), 陈灿(Chen C). 环境科学学报(Acta Scientiae Circum stantiae), 2010, 30(4): 673-701
[17] Linda E. Graham L W W. Algae. New Jersey: Prentice-Hall, Inc., 2000. 97-544
[18] Romera E, Gonzalez F, Ballester A, Blazquez M L, Munoz J A. Crit. Rev. Biotechnol., 2006, 26(4): 223-235
[19] Davis T A, Volesky B, Mucci A. Water Res., 2003, 37(18): 4311-4330
[20] Sari A, Tuzen M. J. Hazard. Mater., 2009, 171(1/3): 973-979
[21] Chen J P, Yang L. Langmuir, 2006, 22(21): 8906-8914
[22] Yang L, Chen J P. Bioresour. Technol., 2008, 99(2): 297-307
[23] Chen J P, Yang L. Ind. Eng. Chem. Res., 2005, 44(26): 9931-9942
[24] Mata Y N, Blazquez M L, Ballester A, Gonzalez F, Munoz T A. J. Hazard. Mater., 2009, 163(2/3): 555-562
[25] Volesky B. Water Res., 2007, 41(18): 4017-4029
[26] Adhiya J, Cai X, Sayre R T, Traina S J. Colloid Surf. A: Physicochem. Eng. Asp., 2002, 210(1): 1-11
[27] Arica M Y, Tuzun I, Yalcin E, Ince O, Bayramoglu G. Process Biochem., 2005, 40(7): 2351-2358
[28] Mehta S K, Gaur J P. Appl. Microbiol. Biotechnol., 2001, 55(3): 379-382
[29] Mohan S V, Ramanaiah S V, Rajkumar B, Sarma P N. J. Hazard. Mater., 2007, 141(3): 465-474
[30] Murphy V, Hughes H, Mcloughlin P. Water Res., 2007, 41(4): 731-740
[31] Kumar Y P, King P, Prasad V. Chem. Eng. J., 2007, 129(1/3): 161-166
[32] Fourest E, Volesky B. Environ. Sci. Technol., 1996, 30(1): 277-282
[33] Chojnacka K, Chojnacki A, Gorecka H. Chemosphere, 2005, 59(1): 75-84
[34] 马静(Ma J).湖南大学硕士论文(Master's Dissertation of Hunan University), 2007
[35] Ghimire K N, Inoue K, Ohto K, Hayashida T. Bioresour. Technol., 2008, 99(1): 32-37
[36] Matos M, Diniz V G, de Abreu C, Knoechelmann A, Da Silva V L. Adsorpt. J. Int. Adsorpt. Soc., 2009, 15(1): 75-80
[37] Rakhshaee R, Giahi M, Pourahmad A. J. Hazard. Mater., 2009, 163(1): 165-173
[38] Southichak B, Nakano K, Nomura M, Chiba N, Nishimura O. Water Sci. Technol., 2009, 59(2): 339-346
[39] Mata Y N, Blazquez M L, Ballester A, Gonzalez F, Munoz J A. J. Hazard. Mater., 2008, 158(2/3): 316-323
[40] Ting Y P, Teo W K, Soh C Y. J. Appl. Phycol., 1995, 7(1): 97-100
[41] 吴燕君(Wu Y J).浙江大学硕士论文(Master's Dissertation of Zhejiang University), 2010
[42] Murphy V, Tofail S, Hughes H, McLoughlin P. Chem. Eng. J., 2009, 148(2/3): 425-433
[43] Murphy V, Hughes H, Mcloughlin P. Chemosphere, 2008, 70(6): 1128-1134
[44] Das B K, Roy A, Koschorreck M, Mandal S M, Wendt-Potthoff K, Bhattacharya J. Water Res., 2009, 43(4): 883-894
[45] 刘静(Liu J), 张道勇(Zhang D Y), 潘响亮(Pan X L), 王立英(Wang L Y). 应用与环境生物学报(Chinese Journal of Applied & Environmental Biology), 2009, 15(3): 347-350
[46] De Philippis R, Sili C, Paperi R, Vincenzini M. J. Appl. Phycol., 2001, 13(4): 293-299
[47] Garcia-Meza J V, Barrangue C, Admiraal W. Environ. Toxicol. Chem., 2005, 24(3): 573-581
[48] Reddy G N, Prasad M. Environ. Exp. Bot., 1990, 30(3): 251-264
[49] Hassler C S, Behra R, Wilkinson K J. Aquat. Toxicol., 2005, 74(2): 139-149
[50] Backor M, Pawlik-Skowronska B, Bud'Ova J, Skowronski T. Plant Growth Regul., 2007, 52(1): 17-27
[51] Cobbett C, Goldsbrough P. Annu. Rev. Plant Biol., 2002, 53: 159-182
[52] Torricelli E, Gorbi G, Pawlik-Skowronska B, Di Toppi L S, Corradi M G. Aquat. Toxicol., 2004, 68(4): 315-323
[53] Morelli E, Cruz B H, Somovigo S, Scarano G. Plant Sci., 2002, 163(4): 807-813
[54] Scarano G, Morelli E. Plant Sci., 2003, 165(4): 803-810
[55] 陈绍勇(Chen S Y),马福俊(Ma F J),龙爱民(You A M),党爱翠(Dang A C), 李春娣(Li C D).环境科学学报(Acta Scientiae Circumstantiae), 2008, 28(5): 873-878
[56] Soldo D, Hari R, Sigg L, Behra R. Aquat. Toxicol., 2005, 71(4): 307-317
[57] Mendoza-Cozatl D G, Moreno-Sanchez R. Biochim. Biophys. Acta-Bioenerg., 2005, 1706(1/2): 88-97
[58] Huang Z Y, Li L P, Huang G L, Yan Q P, Shi B, Xu X Q. Aquat. Toxicol., 2009, 91(1): 54-61
[59] Morris C A, Nicolaus B, Sampson V, Harwood J L, Kille P. Biochem. J., 1999, 338(Part 2): 553-560
[60] Howe G, Merchant S. Plant Physiol., 1992, 98(1): 127-136
[61] Morelli E, Scarano G. Mar. Environ. Res., 2001, 52(4): 383-395
[62] Sabatini S E, Juarez A B, Eppis M R, Bianchi L, Luquet C M, de Molina M. Ecotox. Environ. Safe., 2009, 72(4): 1200-1206
[63] Singh A L, Asthana R K, Srivastava S C, Singh S P. FEMS Microbiol. Lett., 1992, 99(2/3): 165-168
[64] Swift D T, Forciniti D. Biotechnol. Bioeng., 1997, 55(2): 408-418
[65] Nagasaka S, Yoshimura E. Biol. Trace Elem. Res., 2008, 125(3): 286-289
[66] Nishikawa K, Yamakoshi Y, Uemura I, Tominaga N. FEMS Microbiol. Ecol., 2003, 44(2): 253-259
[67] 吴红艳(Wu H Y).微生物学通报(Microbiology), 2003, 30(3): 60-64
[68] Pawlik-Skowronska B. Aquat. Bot., 2003, 75(3): 189-198
[69] Tukaj Z, Bascik-Remisiewicz A, Skowronski T, Tukaj C. Environ. Exp. Bot., 2007, 60(3): 291-299
[70] Nassiri Y, Mansot J L, Wery J, Ginsburgur-Vogel T, Amiar C. Arch Environ. Contam. Toxicol., 1997, 33(2): 147-155
[71] 周文彬(Zhou W B),邱保胜(Qiu B S).湖泊科学(Journal of Lake Science), 2004(03): 265-272
[72] Perez-Rama M, Alonso J A, Lopez C H, Vaamonde E T. Bioresour. Technol., 2002, 84(3): 265-270
[73] Slaveykova V I. Chemosphere, 2007, 69(9): 1438-1445
[74] La Rocca N, Andreoli C, Giacometti G M, Rascio N, Moro I. Photosynthetica, 2009, 47(3): 471-479
[75] Marcano L, Carruyo I M, Montiel X M, Morales C B, de Soto P M. Biol. Trace Elem. Res., 2009, 130(1): 86-93
[76] Al-Homaidan A A. J. Food Agric. Environ., 2008, 6(1): 148-151
[77] Murugesan A G, Maheswari S, Bagirath G. Int. J. Environ. Res., 2008, 2(3): 307-312
[78] Yan H, Pan G. Chemosphere, 2002, 49(5): 471-476
[79] Monteiro C M, Castro P, Malcata F X. World J. Microbiol. Biotechnol., 2009, 25(9): 1573-1578
[80] Schmitt D, Muller A, Csogor Z, Frimmel F H, Posten C. Water Res., 2001, 35(3): 779-785
[81] Kumar R, Goyal D. Indian J. Exp. Biol., 2009, 47(8): 690-694
[82] Doshi H, Ray A, Kothari I L. Biotechnol. Bioeng., 2007, 96(6): 1051-1063
[83] Arunakumara K, Xuecheng Z, Song X. Ceinc Mar., 2007, 33(3): 271-280
[84] Toumi A, Nejmeddine A, El Hamouri B. Water Sci. Technol., 2000, 42(10): 17-21
[85] Adey W H, Luckett C, Smith M. Ecol. Eng., 1996, 7(3): 191-212
[86] De-Bashan L E, Bashan Y. Appl. Environ. Microbiol., 2008, 74(21): 6797-6802
[87] Vijayaraghavan K, Yun Y S. Biotechnol Adv., 2008, 26(3): 266-291
[88] Volesky B, Holan Z R. Biotechnol. Prog., 1995, 11(3): 235-250
[89] Mehta S K, Gaur J P. Crit. Rev. Biotechnol., 2005, 25(3): 113-152
[90] Freitas O, Delerue-Matos C, Boaventura R. J. Hazard. Mater., 2009, 167(1/3): 449-454
[91] Cruz C, Da Costa A, Henriques C A, Luna A S. Bioresour Technol., 2004, 91(3): 249-257
[92] Mehta S K, Gaur J P. Ecol. Eng., 2001, 18(1): 1-13
[93] Klimmek S, Stan H J, Wilke A, Bunke G, Buchholz R. Environ. Sci. Technol., 2001, 35(21): 4283-4288
[94] Vilar V, Botelho C, Boaventura R. J. Hazard. Mater., 2007, 149(3): 643-649
[95] Aksu Z, Donmez G. Process Biochem., 2006, 41(4): 860-868
[96] Karthikeyan S, Balasubramanian R, Iyer C S P. Bioresour. Technol., 2007, 98(2): 452-455
[97] Kumar Y P, King P, Prasad V. J. Hazard. Mater., 2006, 137(2): 1246-1251

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