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化学进展 2008, Vol. 20 Issue (0203): 362-367 前一篇   后一篇

• 综述与评论 •

联吡啶钌修饰电极固相电致化学发光*

陶颖1 林志杰1 陈晓梅1 陈曦1,2**   

  1. (1. 厦门大学化学化工学院化学系现代分析科学教育部重点实验室 厦门 361005;
    2. 厦门大学近海海洋环境科学国家重点实验室 厦门 361005)
  • 收稿日期:2007-04-09 修回日期:2007-05-29 出版日期:2008-03-24 发布日期:2008-03-24
  • 通讯作者: 陈曦

Solid-state Electrochemiluminescence on Tris(2,2'-bipyridine)ruthenium(II) Modified Electrode

Tao Ying1; Lin Zhijie1; Chen Xiaomei1; Chen Xi1,2**   

  1. (1. Key Laboratory of Analytical Sciences of Ministry of Education and Department of Chemistry, Xiamen University, Xiamen 361005, China; 2. State Key Laboratory of Marine Environmental Science, Xiamen University, Xiamen 361005, China)
  • Received:2007-04-09 Revised:2007-05-29 Online:2008-03-24 Published:2008-03-24
  • Contact: Chen Xi
由于电致化学发光(ECL)的连续可测性、高灵敏度、稳定、方法简单,被广泛应用于分子生物学、药学、化学和环保等领域。而将可电化学再生的ECL试剂固定于电极表面, 可获得ECL传感器, 从而减少分析过程中试剂的消耗和简化实验装置。联吡啶钌及其衍生物在电极表面的固定化研究成为ECL研究的重要方向。本文综述了2004年以来联吡啶钌及其衍生物修饰电极的固相ECL的研究进展, 并简要介绍了各种固定方法及其相关的应用情况。
Electrochemiluminescence (ECL) which has been widely used in biological, pharmic, chemical and environmental applications due to its continuance, sensitivity, reproducibility and relative easy to control. The ECL sensor can be assembled by immobilizing electrochemically reproducible ECL reagents on an electrode surface. This approach will reduce the reagents consuming and simplify the detection apparatus. Recently, the studies on the immobilization of tris(2,2'-bipyridine)ruthenium(II) [Ru(bpy)32+] and its derivations have becoming an attractive research field. This review summaries the solid-state ECL development of Ru(bpy)32+ and its derivations since 2004. The approaches for reagent immobilizations as well as the relative applications are also discussed.

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