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化学进展 2007, Vol. 19 Issue (0203): 256-266 前一篇   后一篇

• 综述与评论 •

表面增强荧光研究进展*

吕凤婷1;高莉宁2;房喻1**   

  1. 1. 陕西师范大学化学与材料科学学院 大分子科学陕西省重点实验室 西安 710062;
    2. 陕西师范大学物理学与信息技术学院 西安 710062
  • 收稿日期:2006-04-10 修回日期:2006-08-26 出版日期:2007-03-24 发布日期:2007-03-24
  • 通讯作者: 房喻

Studies of Surface-Enhanced Fluorescence

Lü Fengting1;Zheng Hairong 2,Fang Yu 1**   

  1. 1. Key Laboratory of Macromolecular Science of Shaanxi Province, School of Chemistry and Materials Science,Shaanxi Normal University ,Xi’an 710062, China;
    2. School of Physics and Information Technology, Shaanxi Normal University Xi’an 710062, P. R. China
  • Received:2006-04-10 Revised:2006-08-26 Online:2007-03-24 Published:2007-03-24
  • Contact: Fang Yu
本文比较系统地介绍了金属表面增强荧光现象、产生机理及其应用。粗糙金属和超薄光滑金属表面均可表现出荧光增强效应,但这两种表面增强荧光产生的机理不同,所发出的荧光性质也不同。粗糙金属表面增强荧光的主要原因被认为是加快了处于基质表面附近的荧光物种的辐射衰减过程,而超薄光滑金属表面增强荧光则是激发态荧光物种与金属表面的等离子体耦合共振的结果。与粗糙金属表面增强荧光不同,超薄光滑金属表面增强荧光具有突出的方向性。金属表面增强荧光已经开始在DNA无损检测、荧光共振能量转移免疫分析等领域获得重要应用。
The phenomenon, mechanisms and applications of metallic surfaces-enhanced fluorescence are reviewed. The phenomenon of enhanced fluorescence emission can be observed on both a non-continuous metallic surface and a continuous metallic surface. But the natures of the enhancement are different. The presence of a non-continuous metallic surface can have dramatic effects on the radiative decay rate of a nearby fluorophore.. Above a continuous metallic surface, however,excited fluorophores can couple with surface plasmons, and result in enhanced fluorescence. Compared with the emission near a non-continuous metallic surface, the emission near a continuous metallic surface is highly directional.Furthermore,surface-enhanced fluorescence has found uses in DNA assays, and FRET-based immunoassays.

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[1] 翟彩华, 陈志良, 吕沙沙, 林毅*, 张志淩, 庞代文. 金属增强量子点荧光[J]. 化学进展, 2017, 29(8): 814-823.
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表面增强荧光研究进展*