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化学进展 2006, Vol. 18 Issue (09): 1092-1100 前一篇   后一篇

• 综述与评论 •

多孔膦酸盐的研究进展*

吴宗斌1;田鹏2**;刘中民2;毛宗强1   

  1. 1.清华大学核能与新能源技术研究院 北京 100084;2.中国科学院大连化学物理研究所天然气化工与应用催化研究室  大连 116023
  • 收稿日期:2005-10-19 修回日期:2005-12-27 出版日期:2006-09-24 发布日期:2006-09-24
  • 通讯作者: 田鹏
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Progress in Porous Phosphonates

Zongbin Wu1; Peng Tian2**; Zhongmin Liu2;Zongqiang Mao1   

  1. 1. Institute of Nuclear and New Energy Technology, Tsinghua University, Beijing 100084, China;2. Natural Gas Utilization & Applied Catalysis Laboratory, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China  
  • Received:2005-10-19 Revised:2005-12-27 Online:2006-09-24 Published:2006-09-24
  • Contact: Peng Tian
多孔膦酸盐是一类新型的多孔材料,同时也是一个新兴的研究领域。有机膦配体的多样性和可衍生性赋予这类材料许多独特的性能,因而使其备受关注。本文综述了多孔膦酸盐的合成方法和孔道特征,分析了该领域存在的问题和发展方向。
关键词： 多孔膦酸盐, 合成方法, 孔道特征, 管状形貌
Porous phosphonates are novel porous materials , which have drawn much attention in recent years. The derivable and variety of organophosphorus ligands endow the materials many special properties. The synthetic methods and their characters have been discussed. Precipitation method , melt method , hydrothermal method , solvothermal method ,and template-assisted method have been developed for synthesizing porous phosphonates. Following the principles of coordinate chemistry , these methods give many opportunities for synthesizing a desired structure. Besides the well-known pillared-layered structures and zeolite-type structures , novel tubular morphologies with layered frameworks have been reported recently in some diphosphonates. The tubular morphologies open a new strategy for obtaining porous phosphonates. Up to now , great efforts have been devoted to the porous phosphonates , however , only a few of these compounds are really porous. The removal of the template often leads to the collapse of the structures , which hinders the materials for going further. More works and new ideas should been applied to suppress their drawbacks. Some proposals concerning the key points for porous phosphonates have been presented in the article.
Key words: porous phosphonates, synthetic methods, porous character, tubular morphology

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摘要

多孔膦酸盐的研究进展*