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化学进展 2023, Vol. 35 Issue (7): 1018-1029 DOI: 10.7536/PC221203 前一篇   后一篇

• 综述 •

环境水体中腐殖酸与共存物的相互作用

周春地1, 隋铭皓1,2,*()   

  1. 1 同济大学环境科学与工程学院,污染控制与资源化研究国家重点实验室 上海 200092
    2 上海污染控制与生态安全研究院 上海 200092
  • 收稿日期:2022-12-10 修回日期:2023-04-13 出版日期:2023-07-24 发布日期:2023-06-15
  • 基金资助:
    国家重点研发计划课题(2019YFC0408801)
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Interactions Between Humic Acid and Co-Existing Substances in Aquatic Environments

Chundi Zhou1, Minghao Sui1,2()   

  1. 1 State Key Laboratory of Pollution Control and Resource Reuse, College of Environmental Science and Engineering, Tongji University,Shanghai 200092, China
    2 Shanghai Institute of Pollution Control and Ecological Security,Shanghai 200092, China
  • Received:2022-12-10 Revised:2023-04-13 Online:2023-07-24 Published:2023-06-15
  • Contact: * e-mail: suiminghao.sui@gmail.com
  • Supported by:
    National Key R&D Program of China(2019YFC0408801)

腐殖酸(humic acid, HA)凭借着其赋存特性和独特的化学活性在环境治理领域备受关注。值得注意的是,在共存反应体系中,HA不可避免的与共存物相互作用,进而使反应体系变得复杂,结果导向与预期不同。因此,研究HA与共存物之间的相互作用对于正确理解环境水污染复杂性问题,开发具有协同处理共存物的新型环境功能材料具有重要意义。本文综述了HA参与的共存污染物体系下目标污染物协同/拮抗去除效果,包括无机污染物共存体系、有机污染物共存体系和微生物共存体系。针对HA自身的结构特点和理化性质,系统分析了HA与共存污染物之间的相互作用机理,主要涉及配位作用、静电作用、吸附作用、疏水作用、π-π相互作用和氧化还原作用等。最后,对HA在共存污染体系下目标污染物的去除所面对的挑战和未来的研究方向进行了展望。

关键词： 腐殖酸, 环境水污染, 共存物, 相互作用, 共存体系

Humic acid (HA) has attracted significant attention in the field of environmental remediation due to its occurrence characteristics and unique chemical reactivity. It is worth noting that in co-existing reaction systems, HA inevitably interacts with co-existing substances, making the reaction system complex and leading to unexpected results. Therefore, studying the interaction between HA and co-existing substances is of great significance for a correct understanding of the complexity of environmental water pollution and the development of new environmental functional materials with cooperative treatment of co-existing substances. This article reviews the synergistic/antagonistic removal effects of target pollutants in co-existing pollution systems involving HA, including inorganic co-existing pollutant systems, organic co-existing pollutant systems, and microbial co-existing systems. Based on the structural characteristics and physicochemical properties of HA itself, the interaction mechanisms between HA and co-existing pollutants are systematically analyzed. These mechanisms mainly involve coordination, electrostatic interactions, adsorption, hydrophobic interactions, π-π interactions, and oxidation-reduction reaction (REDOX). Finally, the challenges and future research directions for the removal of target pollutants by HA in co-existing pollution systems are discussed.

Contents

1 Introduction

2 Removal of target contaminant in different co-existing systems

2.1 HA with co-inorganic contaminant system

2.2 HA with co-organic contaminant system

2.3 HA with co-microbial system

2.4 Quantitative comparison of the removal effectiveness in HA co-existing contaminant systems

3 Interaction mechanisms between HA and co-existing contaminant

3.1 HA with co-inorganic contaminant system

3.2 HA with co-organic contaminant system

3.3 HA with co-microbial system

3.4 Characteristics of interaction mechanism in HA co-existing contaminant systems

4 Conclusion and Outlook

Key words: humic acid, environmental water pollution, co-existing substances, interaction, co-existing systems
()
图1 HA的结构单元及官能团种类[8]
Fig.1 Structural units and functional groups of HA[8] Copyright 2011, Springer Nature
图2 HA参与共存体系下污染物的去除效果
Fig.2 The removal synergistic or antagonistic effect of contaminants with HA in co-existing system
表1 重金属氧化还原电位
Table 1 Standard redox potential of heavy metal ions
Cr
(Ⅵ)		 Fe
(Ⅲ)		 Pb
(Ⅱ)		 Cd
(Ⅱ)		 Mg
(Ⅱ)		 Na
(Ⅰ)		 Ca
(Ⅱ)		 K
(Ⅰ)
E0 (Ⅴ) 1.33 0.77 -0.13 -0.40 -2.37 -2.71 -2.87 -2.93
图3 人工腐殖酸稳定高分散零价铁去除铅离子的机制[70]
Fig.3 The possible mechanism of high-dispersion zero-valent iron particles stabilized by artificial humic acid for lead ion removal[70]. Copyright 2019, Elsevier
图4 黑暗条件下腐殖酸介导银离子向银纳米颗粒转化的机制[92]
Fig.4 The possible mechanism of transformation of silver ions to silver nanoparticles mediated by humic acid under dark conditions[92]. Copyright 2019, Elsevier
图5 HA影响MPFs对THIA吸附的机理示意图[101]
Fig.5 Schematic diagram of the possible mechanism of HA affecting the adsorption of THIA on MPFs[101]. Copyright 2022, Elsevier
图6 Gt-HA促进SA类芬顿降解的机制[61]
Fig.6 Potential mechanism of Gt-HA promoted Fenton-like degradation of SA[61]. Copyright 2020, Elsevier
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