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化学进展 2021, Vol. 33 Issue (2): 165-178 DOI: 10.7536/PC201016   后一篇

• 综述 •

基于非富勒烯小分子受体Y6的有机太阳能电池

徐翔1, 李坤1, 魏擎亚1, 袁俊1, 邹应萍1,*()   

  1. 1 中南大学化学化工学院 长沙 410083
  • 收稿日期:2020-10-15 修回日期:2021-01-15 出版日期:2021-02-24 发布日期:2021-01-22
  • 通讯作者: 邹应萍
  • 基金资助:
    国家自然科学基金项目(21875286); 国家重点研发计划(2017YFA0206600)
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Organic Solar Cells Based on Non-Fullerene Small Molecular Acceptor Y6

Xiang Xu1, Kun Li1, Qingya Wei1, Jun Yuan1, Yingping Zou1,*()   

  1. 1 College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China
  • Received:2020-10-15 Revised:2021-01-15 Online:2021-02-24 Published:2021-01-22
  • Contact: Yingping Zou
  • About author:
    * Corresponding author e-mail:
  • Supported by:
    National Natural Science Foundation of China(21875286); National Key Research & Development Projects of China(2017YFA0206600)

随着给/受体材料的不断发展,有机太阳能电池的器件效率不断取得进展。特别是非富勒受体分子Y6的出现,使单结有机太阳能电池的效率突破了15%。Y6已经应用到了有机太阳能电池各个方面并且极大提升了其性能。本综述主要总结了Y6在二元、三元和四元、逐层印刷、柔性、叠层和半透明等有机太阳能电池方面的研究情况,以及基于Y6三线态的有机太阳能电池的进展,最后对Y6的结构优化及在器件领域中的应用进行了展望。

关键词： Y6, 有机太阳能电池, 非富勒烯小分子受体, 效率, 应用

With the development of donor and acceptor materials, the power conversion efficiency(PCE) of organic solar cells(OSCs) has continuously made breakthrough in recent years. Particularly, the emergency of non-fullerene acceptor Y6 has enabled the device efficiency of OSCs over 15%. Y6 has been applied in many aspects and greatly improved its photovoltaic properties. This review focuses on the applications of Y6 in binary, ternary and quaternary, layer-by-layer, flexible, tandem and semitransparent organic solar cells, meanwhile, the future structure optimizations and device applications of Y6 have been outlooked.

Contents

1 Introduction

2 Binary organic solar cells based on Y6

2.1 Polymer donors matching with the Y6 acceptor

2.2 Small molecular donors matching with the Y6 acceptor

3 Ternary and quaternary organic solar cells based on Y6

4 LBL-processed OSCs based on Y6

5 Flexible OSCs based on Y6

6 Tandem OSCs based on Y6

7 Semi-transparent OSCs based on Y6

8 Research on OSCs based on Y6 triplet state

9 Conclusion and outlook

Key words: Y6, organic solar cells, non-fullerene small molecular acceptors, efficiency, applications
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图1 聚合物电子给体材料的结构
Fig. 1 The structures of polymer donors
表1 不同聚合物给体材料与Y6共混的二元有机太阳能电池器件的光伏性能
Table 1 The photovoltaic performance of binary organic solar cells based on different polymer donors and Y6
Active layer Voc(V) Jsc(mA/cm2) FF PCE(%) ref
PTQ10:Y6 0.83 26.65 0.75 16.53 35
PM7:Y6 0.90 25.64 0.74 17.04 36
PBFTz:Y6 0.91 13.00 0.59 6.90 37
PM1:Y6 0.87 25.90 0.78 17.6 37
PM2:Y6 0.90 24.90 0.69 15.5 37
P2F-EHp:Y6 0.81 26.68 0.74 16.02 38
PTzBI-dF:Y6 0.85 26.33 0.76 16.8 40
J52-FS:Y6 0.81 22.92 0.57 10.58 41
PE2:Y6 0.83 23.24 0.70 13.50 41
PE4:Y6 0.84 23.77 0.75 14.02 42
Pt-PSFTZ:Y6 0.81 26.45 0.76 16.35 43
D16:Y6
D18:Y6 		0.85
0.86 		25.41
27.70 		0.75
0.77 		16.72
18.22 		44
45
图2 小分子给体材料的结构
Fig. 2 The structures of small molecular donors
表2 不同小分子给体材料与Y6共混的二元有机太阳能电池器件的光伏性能
Table 2 The photovoltaic performance of binary organic solar cells based on different small molecular donors and Y6
Active layer Voc(V) Jsc(mA/cm2) FF PCE(%) ref
BTEC-1F:Y6 0.87 21.21 0.61 11.33 52
BTEC-2F:Y6 0.85 21.55 0.72 13.34 52
BTR-Cl:Y6 0.86 24.17 0.66 13.60 53
ZR1:Y6 0.86 24.34 0.68 14.34 55
SM1-F:Y6 0.87 23.25 0.70 14.07 56
BTTzR:Y6 0.88 23.20 0.68 13.90 57
图3 有机太阳能电池中第三或第四组分的化学结构
Fig. 3 The chemical structures of the third or fourth components in organic solar cells
表3 基于Y6的三元和四元有机太阳能电池器件的光伏性能
Table 3 The photovoltaic performance of ternary and quaternary organic solar cells based on Y6 acceptor
Active layer Voc(V) Jsc(mA/cm2) FF PCE(%) ref
PM6:Y6:PC61BM 0.85 25.40 0.77 16.50 87
PM6:Y6:IDIC 0.87 25.39 0.75 16.51 85
PM6:Y6:3TP3T-4F 0.85 25.90 0.75 16.70 88
PM6:Y6:DRTB-T-C4 0.85 24.79 0.81 17.13 89
PM6:Y6:IDIC:PC71BM
PM6:Y6:PC71BM:PhI-Se 		0.87
0.85 		26.19
26.30 		0.75
0.77 		17.07
17.20 		96
31
PM6:PM7:Y6:PC71BM 0.86 26.55 0.79 18.07 97
图4 可折叠柔性OSC的光伏特性:(A)柔性OSC的器件结构;(B)在ITO/PET和PEDOT上制备柔性OSCs的J-V特性:三种环保酸处理的PEDOT:PSS/PET;(C) m-PEDOT制备的柔性OSCs的最佳J-V特性:柠檬酸处理的PEDOT:PSS/PET(插图对应20个单个器件PCE计数的直方图分布);(D) 最近关于柔性OSCs的PCE值的散点图报告[116]
Fig. 4 Photovoltaic characteristics of folding-flexible OSCs.(A) Device structure of the flexible OSC.(B) J-V characteristics of flexible OSCs fabricated on ITO/PET and PEDOT:PSS/PET with three eco-friendly acid treatments.(C) Optimal J-V characteristics of flexible OSCs fabricated on m-PEDOT:PSS/PET with citric acid treatments(insert is corresponding histogram distribution of PCE counts for 20 individual devices).(D) Recent scatterplot report for PCE values of flexible OSCs. Reproduced with permission[116]. Copyright 2020, Cell.
图5 生动多彩的ST-OSCs:(a)彩色OSCs的结构和厚度;(b)PM6、Y6和Bis-FIMG的化学结构;(c)双层TEs: glass/ITO/Ag(15 nm)和glass/ITO/Bis-FIMG/Ag(15 nm)的透射光谱,绿色曲线表示人眼对光反应;(d)基于CIE 1931模拟的带有F-P电极的彩色ST-OSCs颜色坐标[146]
Fig. 5 Vividly colorful ST-OSCs.(a) Structure and layer thickness of colorful OSCs.(b) Chemical structures of PM6, Y6, and Bis-FIMG.(c) Transmittance spectra of double-layered TEs: glass/ITO/Ag(15 nm) and glass/ITO/Bis-FIMG/Ag(15 nm); green curve for photopic response of human eye.(d) Simulated color coordinates of colorful ST-OSCs with F-P electrodes on the CIE 1931. Reproduced with permission[146] Copyright 2020, American Chemical Society.
图6 三线态非富勒烯受体材料化学结构图
Fig. 6 Structure diagram of triplet non-fullerene acceptors
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