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化学进展 2020, Vol. 32 Issue (7): 989-1002 DOI: 10.7536/PC191202 前一篇   后一篇

• 综述 •

印迹复合膜

汪润田1,2, 柳春丽1,2,**(), 陈振斌1,2,**()   

  1. 1. 兰州理工大学 材料科学与工程学院 兰州 730050
    2. 兰州理工大学 省部共建有色金属先进加工与再利用国家重点实验室 兰州 730050
  • 收稿日期:2019-12-05 出版日期:2020-07-24 发布日期:2020-07-10
  • 通讯作者: 柳春丽, 陈振斌
  • 基金资助:
    沈阳材料科学国家研究中心-有色金属加工与再利用国家重点实验室联合基金(18LHZD003); 沈阳材料科学国家研究中心-有色金属加工与再利用国家重点实验室联合基金(18LHPY004)

Imprinted Composite Membranes

Runtian Wang1,2, Chunli Liu1,2,**(), Zhenbin Chen1,2,**()   

  1. 1. College of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou 730050, China
    2. State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals, Lanzhou University of Technology, Lanzhou 730050, China
  • Received:2019-12-05 Online:2020-07-24 Published:2020-07-10
  • Contact: Chunli Liu, Zhenbin Chen
  • About author:
    ** e-mail: (Chunli Liu);
    (Zhenbin Chen)
  • Supported by:
    joint fund between Shenyang National Laboratory for Materials Science and State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals(18LHZD003); joint fund between Shenyang National Laboratory for Materials Science and State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals(18LHPY004)

印迹复合膜由于兼具分离膜的高效分离性能与印迹聚合物的特异识别性分离性能,可实现对目标物质的精准分离而引起极大关注,相关研究报道也逐年增加。然而,尚无关于印迹复合膜相关研究进展的总结及对存在问题和未来发展趋势的分析和展望。本文首先总结了印记复合膜的研究发展历程,随后从印迹复合膜制备技术的研究进展出发,根据印迹复合膜的结构,将其分为单层结构印迹复合膜、双层结构印迹复合膜、多层结构印迹复合膜、基于三维大孔基底的印迹复合膜以及智能印迹复合膜,并分别综述了各类印迹复合膜的结构特征、制备方法、识别/分离性能以及它们各自存在的问题,最后对其未来发展方向进行展望。

Imprinted composite membranes(IcMs) not only possess the efficient separation performance of membranes, but also possess the selective separation performance of imprinted polymers, which have attracted extensive attention all over the world for their well and precise separation property for target substances and high membrane flux. However, the research progress on IcMs has not been summarized yet, and problems existed in research process and the future perspective of IcMs are not analyzed and forecast. This paper summarizes the research and development process of IcMs and the research progress in preparation technology of IcMs, then classify IcMs according to their structure to several categories, namely, IcMs of a single-layer structure, IcMs of a dual-layer structure, IcMs of a multi-layer structure, IcMs of 3D macroporous structure and IcMs with smart sensing and separation properties. Finally, the preparation methods, structural characteristics and identification/separation properties of IcMs, and the potential problems coupled with those aspects are summarized and a future developing direction of this field is prospected.

Contents

1 Introduction

2 Imprinted membranes

2.1 History of imprinted membranes

2.2 Recognition mechanism and transfer mechanism of imprinted composite membranes

3 Classification of imprinted composite membranes based on structural differences

3.1 Single-layer structure imprinted composite membranes

3.2 Dual-layer structure imprinted composite membranes

3.3 Multi-layer structure imprinted composite membranes

3.4 3D macroporous imprinted composite membranes

4 Smart imprinted composite membranes

4.1 Switch-smart imprinted composite membrane

4.2 Integrated-smart imprinted composite membrane

5 Conclusion and outlook

()
图1 印迹过程及其识别机理示意图
Fig.1 The preparation route of imprinted separation layer and recognition mechanism
图2 印迹膜溶解-扩散模型[31]
Fig.2 Mass transfer mechanism solution-diffusion model of imprinting membranes[31] Copyright 2001, Elsevier
图3 “门”模型[30]
Fig.3 “Gate”model[30] Copyright 1999, Elsevier
图4 底物中模板在印迹复合膜中的扩散柱坐标图[34]
Fig.4 Schedule of diffusion of template imprinting composite membrane[34]
图5 氯唑西林印迹复合膜的制备过程示意图[39]
Fig.5 Schematic illustration of constructing IcMs for Cloxicillin[39]. Copyright 2018, Elsevier
图6 D-色氨酸制备过程示意图[10]
Fig.6 Schematic illustration of constructing IcMs for D-Tryptophan[10].Copyright 2017, Elsevier
图7 铜离子印迹复合膜的制备过程示意图[13]
Fig.7 Schematic illustration of constructing IcMs for Cu2+[13]. Copyright 2018, Elsevier
图8 青蒿素印迹复合膜的制备过程示意图[46]
Fig.8 Schematic illustration of constructing IcMs for artemisinin[46]. Copyright 2014, Elsevier
图9 布洛芬印迹复合膜制备示意图[47]
Fig.9 Schematic illustration of constructing IcMs for ibuprofen[47]. Copyright 2018, Elsevier
图10 恩诺沙星的印迹复合膜制备示意图[48]
Fig.10 Schematic illustration of constructing IcMs for enrofloxacin[48]. Copyright 2019, Elsevier
图11 青蒿素印迹复合膜的制备过程示意图[51]
Fig.11 Schematic illustration of constructing IcMs for artemisinin[51]. Copyright 2016, Wiley
图12 Mo(Ⅵ)印迹复合膜制备示意图[52]
Fig.12 Schematic illustration of constructing IcMs for Mo(Ⅵ)[52].Copyright 2016, Elsevier
图13 诺氟沙星印迹复合膜的制备示意图[53]
Fig.13 Schematic illustration of constructing IcMs for norfloxacin[53]. Copyright 2018, Elsevier
图14 诺氟沙星印迹复合膜制备示意图[54]
Fig.14 Schematic illustration of constructing IcMs for norfloxacin[54].Copyright 2017, Royal Society of Chemistry
图15 布洛芬印迹复合膜制备示意图[55]
Fig.15 Schematic illustration of constructing IcMs for ibuprofen[55].Copyright 2018, Elsevier
图16 依诺沙星印迹复合膜制备示意图[56]
Fig.16 Schematic illustration of constructing IcMs for enoxacin[56].Copyright 2019, Elsevier
图17 青蒿素印迹复合膜的制备过程示意图[57]
Fig.17 Schematic illustration of constructing IcMs for artemisinin[57]. Copyright 2015, Elsevier
图18 Li+的印迹复合膜制备示意图[58]
Fig.18 Schematic illustration of constructing IcMs for Li+[58]. Copyright 2018, Elsevier
图19 卵清蛋白印迹复合膜的制备示意图[59]
Fig.19 Schematic illustration of constructing IcMs for ovalbumin[59]. Copyright 2015, Wiley
图20 青蒿素的印迹复合膜的制备示意图[60]
Fig.20 Schematic illustration of the synthesis of IcMs for artemisinin[60]. Copyright 2019, America Chemistry Society
图21 Li+的印迹复合膜的制备示意图[61]
Fig.21 Schematic illustration of the sythesis of IcMs for Li+[61]. Copyright 2019, Elsevier
图22 Pd2+的IcMs制备过程示意图[62]
Fig.22 Scheme for the preparation of IcMs for Pd2+[62]. Copyright 2020, Elsevier
图23 大黄素的IcMs制备过程示意图[63]
Fig.23 Scheme for the preparation of IcMs for emodin[63]. Copyright 2019, Elsevier
图24 Dy3+的IcMs制备过程示意图[64]
Fig.24 Scheme for the preparation of IcMs for Dy3+[64]. Copyright 2017, Elsevier
图25 环丙沙星的印迹复合膜制备示意图[23]
Fig.25 Scheme for the preparation of IcMs for ciprofloxacin[23]. Copyright 2017, Elsevier
图26 Eu3+的印迹复合膜制备示意图[66]
Fig.26 Scheme for the preparation of IcMs for Eu3+[66]. Copyright 2018, Elsevier
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