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化学进展 2019, Vol. 31 Issue (4): 571-579 DOI: 10.7536/PC180823 前一篇   后一篇

• •

多巴胺功能材料在水污染控制中的应用

陈贺1, 张帅其1, 赵致雪1, 刘萌1, 张庆瑞1,2,**()   

  1. 1. 燕山大学环境与化学工程学院 秦皇岛 066004
    2. 河北省应用化学重点实验室 秦皇岛 066004
  • 收稿日期:2018-08-28 出版日期:2019-01-15 发布日期:2019-01-14
  • 通讯作者: 张庆瑞
  • 作者简介:
  • 基金资助:
    国家自然科学基金项目资助(51578476); 国家自然科学基金项目资助(21876145)
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Application of Dopamine Functional Materials in Water Pollution Control

He Chen1, Shuaiqi Zhang1, Zhixue Zhao1, Meng Liu1, Qingrui Zhang1,2,**()   

  1. 1. School of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao 066004, China
    2. Key Laboratory of Applied Chemistry of Hebei Province, Qinhuangdao 066004, China
  • Received:2018-08-28 Online:2019-01-15 Published:2019-01-14
  • Contact: Qingrui Zhang
  • About author:
    ** E-mail:
  • Supported by:
    Fund:The work was supported by the National Natural Science Foundation of China(51578476); Fund:The work was supported by the National Natural Science Foundation of China(21876145)

多巴胺又名4-(2-乙氨基)-苯-1,2-二酚,具有官能团丰富,吸附位点多以及良好的生物相容性等众多优势,近年来,利用多巴胺研制纳米复合功能材料及环境应用是重要研究方向之一。本文从多巴胺结构特性以及自聚组装机理入手,介绍了将聚多巴胺涂布于不同基底材料进行改性,总结性能优异的多巴胺纳米复合材料的制备方法及在污水处理方面的应用进展及应用前景。

关键词： 多巴胺, 纳米材料, 重金属, 有机物, 吸附

Dopamine, known as 4-(2-ethylamino)-benzene-1, 2-diphenol, exhibits abundance in functional groups and active sites for adsorption, as well as good biocompatibility. Recently, an important research area has been emerging using dopamine based nanocomposite for environmental remediation. In this paper, the structural characteristics of dopamine and the mechanism of self-polymerization are introduced, and the polydopamine coating onto various substrates and the relative applications for wastewater treatment are discussed.

Key words: dopamine, nanomaterials, heavy metal, organic matter, adsorption
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图1 不同儿茶酚类的结构图[14]
Fig. 1 Structure diagram of different catechols[14]. Copyright 2017, Wiley.
图2 不同PDA结构[18]
Fig. 2 Different PDA structures[18]. Copyright 2013, ACS.
图3 多巴胺在水溶液中的反应路线[23]
Fig. 3 The reaction route of dopamine in aqueous solution[23]. Copyright 2015, Elsevier.
图4 CuSO4/H2O2为氧化剂制备PDA膜[36]
Fig. 4 Preparation of PDA Membrane by CuSO4 / H2O2 as Oxidant[36]. Copyright 2017, ACS.
图5 多巴胺与不同材料基体发生共沉积时的相互作用[41]
Fig. 5 Interaction of dopamine with co-deposition of different material matrices[41]. Copyright 2018, Wiley.
图6 石墨烯水凝胶吸附污水效果图[52]
Fig. 6 Effect of PDA-GH on adsorption of sewage[52].Copyright 2013, ACS.
图7 通过PDA化学介导的SET-LRP的AO功能化MNPs合成示意图[56]
Fig. 7 Illustration of the synthetic procedure of AO-functio-nalized MNPs by SET-LRP mediated by PDA chemistry[56].Copyright 2016, RSC.
图8 (a)Fe3O4@PDA-Ag核/壳纳米球制备示意图;(b)Fe3O4@PDA-Ag核/壳纳米球吸附MB连续紫外-可见光谱图[64]
Fig. 8 (a)Schematic diagram of preparation of Fe3O4 @PDA-Ag core/shell nanospheres;(b)Successive UV-vis absorption spectra of MB aqueous solution in the presence of Fe3O4@PDA-Ag core-shell microspheres[64].Copyright 2014, ACS.
图9 Ag纳米颗粒载入PDA涂覆的3D-IO结构的模板示意图[76]
Fig. 9 Schematic procedure of fabricating Ag nanoparticle-incorporated free-standing membranes using a template of a PDA-coated 3D-IO structure[76]. Copyright 2016, ACS.
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