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化学进展 2019, Vol. 31 Issue (2/3): 322-336 DOI: 10.7536/PC180741 前一篇   后一篇

• •

高流明密度激光照明用光转换材料

康健1, 张乐1,**(), 甄方正1, 单迎双1, 马跃龙1,2, 陈浩1,**()   

  1. 1. 江苏师范大学物理与电子工程学院 江苏省先进激光材料与器件重点实验室 徐州 221116
    2. 江苏大学机械工程学院 镇江 212013
  • 收稿日期:2018-07-30 出版日期:2019-02-15 发布日期:2018-12-20
  • 通讯作者: 张乐, 陈浩
  • 基金资助:
    国家自然科学基金项目(61775088); 国家自然科学基金项目(51402133); 国家自然科学基金项目(61603160); 江苏高校优势学科建设工程资助项目(PAPD); 江苏省重点研发计划(BE2018062); 江苏省研究生科研与实践创新项目(KYCX18_2096); 江苏省研究生科研与实践创新项目(KYCX18_2097); 江苏省研究生科研与实践创新项目(KYCX18_2098); 江苏省研究生科研与实践创新项目(KYCX18_2099); 徐州市科技创新专项资金项目(KC16GZ014); 徐州市科技创新专项资金项目(KC16HQ236); 徐州市科技创新专项资金项目(KC16HQ237)
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Light-Conversion Materials for High-Lumen Density Laser Illumination

Jian Kang1, Le Zhang1,**(), Fangzheng Zhen1, Yingshuang Shan1, Yuelong Ma1,2, Hao Chen1,**()   

  1. 1. Jiangsu Key Laboratory of Advanced Laser Materials and Devices, School of Physics Electronic Engineering, Jiangsu Normal University, Xuzhou 221116, China
    2. School of Mechanical Engineering, Jiangsu University, Zhenjiang 212013, China
  • Received:2018-07-30 Online:2019-02-15 Published:2018-12-20
  • Contact: Le Zhang, Hao Chen
  • About author:
    ** E-mail: (Le Zhang);
    (Hao Chen)
  • Supported by:
    National Natrual Science Foundation of China(61775088); National Natrual Science Foundation of China(51402133); National Natrual Science Foundation of China(61603160); Priority Academic Program Development of Jiangsu Higher Education Institutions(PAPD); Key R&D Plan of Jiangsu Province(BE2018062); Graduate Students Scientific Research and Practical Innovation Projects of Jiangsu Province(KYCX18_2096); Graduate Students Scientific Research and Practical Innovation Projects of Jiangsu Province(KYCX18_2097); Graduate Students Scientific Research and Practical Innovation Projects of Jiangsu Province(KYCX18_2098); Graduate Students Scientific Research and Practical Innovation Projects of Jiangsu Province(KYCX18_2099); Special Fund for Science and Technology of Xuzhou(KC16GZ014); Special Fund for Science and Technology of Xuzhou(KC16HQ236); Special Fund for Science and Technology of Xuzhou(KC16HQ237)

激光白光光源具有亮度高、响应速度快和传输距离远等优点,在汽车照明、显示、工业照明及高铁舰船等远程照明领域获得广泛应用。然而,随着流明密度不断增加,对光转换材料提出了更高的要求。本文对激光照明用粉体、单晶、玻璃、陶瓷等光转换材料的国内外研究进展进行了综述;简要分析了当前光转换材料温度猝灭现象的主要原因;提出了实现高流明密度激光照明应用所需要解决的关键问题,最后对其发展趋势进行了展望。

关键词： 激光照明, 荧光陶瓷, 高流明密度, 高发光效率

Laser-based white-light source has the advantages of high brightness, fast response and far transmission distance. It is widely used in automotive lighting, display, industrial lighting, and remote lighting fields such as high-speed rail and ships. However, with the high lumen density of laser illumination source, higher requirements are proposed for the light-conversion materials. In this review, the research progress of light-converting materials such as powder, single crystal, glass and ceramics for laser illumination in recent years is reviewed. Then, the main causes of temperature quenching of current light-conversion materials are briefly analyzed. Finally, several key problems to be urgently solved are highlighted for the application of high-lumen density laser illumination, and its development trend is prospected.

Key words: laser illumination, florescent ceramic, high-lumen density, high luminous efficiency
()
图1 Ce:YAG荧光粉体在激光激发下获得的发光光谱和 “散斑”(内插图)[30]
Fig. 1 The luminescence spectrum and speckle(inset) of Ce:YAG phosphors under laser excitation[30]. Copyright 2013, AIP Advances.
图2 SiO2-Ce:YAG厚膜在(a)不同基底下的归一化强度以及(b)在氧化铝基底下不同厚度厚膜的发光强度[40]
Fig. 2 The normalized intensity of SiO2-Ce:YAG thick films under(a) different substrates and(b) alumina substrate with different thickness[40]. Copyright 2017, Elsevier
图3 (a)基于透明基底[41]及(b, c)反射基底[43]的远程激发荧光体装置
Fig. 3 A remote excitation fluorescence device based on transparent substrate(a)[41]and reflection substrate(b, c)[43]
图4 不同温度下(a)Ce:LuAG单晶、(b)多晶的发光强度[45]
Fig. 4 The luminous intensity of(a) Ce:LuAG single crystal and(b) polycrystalline at different temperatures[45]. Copyright 2017, Elsevier
图5 (a)四种石榴石单晶的发光光谱及其(b)内部量子效率随温度的变化[50]
Fig. 5 The luminescence spectra of four garnet single crystals(a) and their internal quantum efficiencies with the variation of working temperature(b)[50]. Copyright 2018, Springer
图6 PIG(phosphors-in-glass)的显微结构和光学特性:(a)初始玻璃的SEM;(b)初始荧光粉的SEM;(c)PIG的激光显微镜图像;(d)PIG的光学特性[53]
Fig. 6 The microstructural characterization and optical properties of PIG:(a) SEM image of glass frits;(b) SEM image of phosphor powders;(c) laser microscopy image of PIG;(d) the optical properties of PIG[53]. Copyright 2015, Royal Society of Chemistry
图7 Ce:YAG荧光陶瓷激发功率密度和光通量关系[59]
Fig. 7 Power density versus luminous flux of Ce:YAG fluorescence ceramics[59]. Copyright 2018, Web of Science
表1 Ce:YAG荧光陶瓷和传统粉体封装性能比较[59]
Table 1 Properties between Ce:YAG fluorescent ceramic and traditional powders packaging[59]
Types CCT CRI CIE Current
(mA)		 lm/μm
x y
Powders 9938 53.9 0.289 0.271 400 1.285
Ceramics 6052 54.2 0.321 0.332 400 2.691
图8 气孔和第二相作为散射中心提高光提取示意图[62]
Fig. 8 The diagram of the pores and the second phase used as scattering centers to improve the luminous efficiency[62].
图9 不同探测器的角度获得的不同颜色质量的光源[63]
Fig. 9 Sources with different color qualities can be obtained with different detector angles[63]. Copyright 2016, Royal Society of Chemistry
图10 荧光陶瓷在不同表面处理方式下的SEM:(a)镜面抛光;(b)未抛光;(c)热刻蚀以及(d)表面经过不同方式处理获得的发光光谱[66]
Fig. 10 SEM images of(a) mirror polished,(b) unpolished,(c) thermally etched and Luminescence spectra(d) obtained by surface treatment in different ways[66]. Copyright 2018, Elsevier
图11 Al2O3-Ce:YAG复相陶瓷和Ce:YAG单晶的在空间上光强的分布:(a)陶瓷;(b)单晶;在激光激发下实物图:(c)陶瓷;(d)单晶[67]
Fig. 11 Normalized emission intensity for(a) a Al2O3-Ce:YAG ceramic composite and(b) a roughened Ce:YAG single crystal and their illuminant circs in the photograph:(c) fluorescent ceramics;(d) single crystals[67]. Copyright 2018, American Chemical Society
图12 不同功率密度下,Ce:LuAG陶瓷发射光谱[62]
Fig. 12 Emission spectra of Ce:LuAG ceramics at different power densities[62]. Copyright 2018, Elsevier
图13 激光直写功率为65 MW/cm2时6H-SiC在325 nm激发下发射类标准白光光谱[77]
Fig. 13 Pseudo-standard white light spectrum of 6H-SiC obtained when excited at 325 nm and laser direct write power is 65 MW/cm2[77]. Copyright 2018, Web of Science
图14 Ce:AlN陶瓷在激光激发下的类标准白光光谱[79]
Fig. 14 Pseudo-standard white light spectrum obtained from Ce:AlN ceramics excited by laser[79]. Copyright 2016, AIP Advances.
图15 在不同Ce3+浓度下,Ce:YAG荧光粉体在不同温度下的荧光寿命[91]
Fig. 15 Temperature dependence of the fluorescence lifetime for Ce:YAG at different Ce3+ concentrations[91]. Copyright 2009, American Chemical Society
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