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化学进展 2017, Vol. 29 Issue (12): 1446-1461 DOI: 10.7536/PC170744 前一篇   后一篇

• 综述 •

大气污染物中人工放射性铯-钚-铀同位素示踪技术的发展与应用

欧阳洁1,2,3, 杨国胜4, 马玲玲1,3, 罗敏1,3, 徐殿斗1,3*   

  1. 1. 中国科学院高能物理研究所 北京 100049;
    2. 中国科学院大学 北京 100049;
    3. 北京市射线成像技术与装备工程技术研究中心 北京 100049;
    4. 日本弘前大学辐射医疗综合研究所 日本弘前市 036-8564
  • 收稿日期:2017-07-31 修回日期:2017-10-13 出版日期:2017-12-15 发布日期:2017-11-15
  • 通讯作者: 徐殿斗,xudd@ihep.ac.cn E-mail:xudd@ihep.ac.cn
  • 基金资助:
    国家自然科学基金项目（No.11545001，11575210，91643206）和中国科学院高能物理研究所创新基金项目（No.Y7545110U2）资助
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Development and Application of Fingerprints of Radioactive Cesium-Plutonium-Uranium Isotopes as Tracers in Air Pollution

Jie Ouyang1,2,3, Guosheng Yang4, Lingling Ma1,3, Min Luo1,3, Diandou Xu1,3*   

  1. 1. Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China;
    2. University of Chinese Academy of Sciences, Beijing 100049, China;
    3. Beijing Engineering Research Center of Radiographic Techniques and Equipment, Beijing 100049, China;
    4. Department of Radiation Chemistry, Institute of Radiation Emergency Medicine, Hirosaki University, 66-1, Hirosaki 036-8564, Japan
  • Received:2017-07-31 Revised:2017-10-13 Online:2017-12-15 Published:2017-11-15
  • Supported by:
    The work was supported by the National Natural Science Foundation of China (No.11545001, 11575210, 91643206) and the Institute of High Energy Physics, Chinese Academy of Sciences Innovation Fund (No.Y7545110U2).
近年来，我国雾霾形式的大气污染频发，严重影响国人健康和社会经济发展。目前所知，我国大气污染物来源复杂且具有独特性，其源解析研究对于大气污染物防治具有重要意义。随着放射性同位素示踪技术的发展，利用其研究大气污染物来源的问题备受关注。放射性同位素示踪技术及其在环境科学领域中的应用研究已取得了较大成就，特别是利用放射性同位素示踪环境污染物来源等方面。目前已有多种放射性同位素被用于大气污染物源解析研究。本文简要介绍了人工放射性核素铯、钚和铀同位素比值在大气污染物源解析研究中的发展和应用，并提出了存在的问题以及未来的发展趋势，希望进一步推动放射性同位素示踪技术在环境科学特别是在大气污染防治中的应用和发展。
关键词： 大气污染, 污染物源解析, 放射性铯同位素示踪, 放射性钚同位素示踪, 放射性铀同位素示踪
Recently, air pollution occurs frequently in China mainly in the form of haze, which poses great risks to human health and obstacles to social and economic development. It is well known that the sources of China's air pollution are complicated and unique, and the source identification of air pollutants is one of key points in air pollution prevention. With the development of radioisotope tracer technology, its utilization in the source identification of air pollutants has attracted increasing attention. Recently, this technology has obtained great achievements in environmental science, especially in the source identification of environmental pollutants. A variety of radioactive isotopes have been used in the source identification of air pollutants. The article presents a brief overview on the development and application of isotopes of radioactive cesium, plutonium and uranium in the source apportionment of air pollutants, as well as the existing problems and their future prospect.
Contents
1 Introduction
2 Advances of radioisotope on air pollutant tracing study
2.1 Research progress of cesium isotope tracing
2.2 Research progress of plutonium isotope tracing
2.3 Research progress of uranium isotope tracing
3 Radioactive isotope fingerprints of air pollution sources
4 Conclusion and outlook
Key words: air pollution, pollutant source identification, radioactive cesium fingerprints, radioactive plutonium fingerprints, radioactive uranium fingerprints

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