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化学进展 2017, Vol. 29 Issue (9): 1115-1126 DOI: 10.7536/PC170443 前一篇   后一篇

• 综述 •

铋系光催化剂去除环境污染物

丁星1,2, 杨祥龙1, 熊中亮1, 陈浩1*, 张礼知2*   

  1. 1. 华中农业大学理学院 武汉 430070;
    2. 华中师范大学化学学院 环境与应用化学研究所 农药与化学生物学教育部重点实验室 武汉 430079
  • 收稿日期:2017-04-26 修回日期:2017-07-18 出版日期:2017-09-15 发布日期:2017-09-05
  • 通讯作者: 张礼知,e-mail:zhanglz@mail.ccnu.edu.cn;陈浩,e-mail:hchenhao@mail.hzau.edu.cn E-mail:zhanglz@mail.ccnu.edu.cn;hchenhao@mail.hzau.edu.cn
  • 基金资助:
    国家自然科学基金项目（No.21607047，51572101）和湖北省自然科学基金项目（No.2016CFB193）资助
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Environment Pollutants Removal with Bi-Based Photocatalysts

Xing Ding1,2, Xianglong Yang1, Zhongliang Xiong1, Hao Chen1*, Lizhi Zhang2*   

  1. 1. College of Science, Huazhong Agricultural University, Wuhan 430070, China;
    2. Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, Institute of Environmental & Applied Chemistry, College of Chemistry, Central China Normal University, Wuhan 430079, China
  • Received:2017-04-26 Revised:2017-07-18 Online:2017-09-15 Published:2017-09-05
  • Supported by:
    The work was supported by the National Natural Science Foundation of China (No. 21607047, 51572101) and the Natural Science Foundation of Hubei Province (No. 2016CFB193).
铋系半导体材料是近年来研究较热的一类新型光催化剂，因其具有独特的层状结构和合适的禁带宽度，而表现出了良好的太阳光催化性能，在环境污染物去除方面展现出极大的潜力。本文综述了近年来铋系光催化剂（氧化铋、硫化铋、钨酸铋、钼酸铋、钒酸铋、卤氧化铋等）在环境污染物去除方面的最新研究进展，介绍了几类常见的铋系半导体材料及其制备方法，归纳和总结了铋系光催化剂在大气净化、有机废水处理、重金属离子处理和杀菌等方面的应用，同时对今后铋系光催化剂在环境污染去除方面的应用进行了展望。
关键词： 铋系半导体, 可见光, 光催化, 环境污染物
In recent years, Bi-based semiconductor materials have gained considerable attention. Their unique layered structure and suitable band gap endow them with superior visible light photocatalytic activities, which is promising in environment pollutants removal. This article mainly reviews the recent advances in environment contaminants removal with Bi-based photocatalysts. We first introduce several well-known Bi-based semiconductor materials and their preparation methods, and then summarize their applications for air purification, organic wastewater treatment, heavy metal ions removal, disinfection, and finally discuss the major problems in the field of bismuth-based photocatalysts, and prospect their further development in the future.
Contents
1 Introduction
2Bi-based photocatalysts and their preparation methods
2.1 Unary Bi-based photocatalysts
2.2 Binary Bi-based photocatalysts
2.3 Bismuth oxyhalides
3 Environment pollutants removal with Bi-based photocatalysts
3.1 Air purification
3.2 Refractory organic wastewater treatment
3.3 Inorganic wastewater treatment
3.4 Disinfection
4 Conclusion
Key words: Bi-based semiconductors, visible light, photocatalysis, environment pollutants

中图分类号: 

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摘要

铋系光催化剂去除环境污染物