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化学进展 2015, Vol. 27 Issue (2/3): 157-167 DOI: 10.7536/PC140821 前一篇   后一篇

• 综述与评论 •

光响应固体表面的浸润性调控

詹媛媛1, 刘玉云1, 吕久安1, 赵勇2, 俞燕蕾*1   

  1. 1. 复旦大学材料科学系聚合物分子工程国家重点实验室 上海 200433;
    2. 北京航空航天大学化学与环境学院 北京 100191
  • 收稿日期:2014-08-01 修回日期:2014-10-01 出版日期:2015-03-15 发布日期:2014-12-22
  • 通讯作者: 俞燕蕾 E-mail:ylyu@fudan.edu.cn
  • 基金资助:

    国家自然科学基金重点项目(No.21134003),国家自然科学基金面上项目(No.21273048)和国家杰出青年科学基金(No.51225304)资助

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导出 被引次数 ( 2 | 1 )

Photoresponsive Surfaces with Controllable Wettability

Zhan Yuanyuan1, Liu Yuyun1, Lv Jiuan1, Zhao Yong2, Yu Yanlei*1   

  1. 1. State Key Laboratory of Molecular Engineering of Polymers, Department of Materials Science, Fudan University, Shanghai 200433, China;
    2. School of Chemistry and Environment, Beihang University, Beijing 100191, China
  • Received:2014-08-01 Revised:2014-10-01 Online:2015-03-15 Published:2014-12-22
  • Supported by:

    The work was supported by the State Key Program of National Natural Science of China(No. 21134003), the National Natural Science Foundation of China(No. 21273048), and the National Science Foundation for Distinguished Young Scholars of China (No. 51225304).

物质表面能和表面微观结构是影响物质浸润性的两大主要因素,表面能决定了平滑表面的液体接触角,而表面微观结构影响表面的浸润性。在受到外界刺激时,物质表面可发生表面能和表面微观结构的变化,从而实现表面浸润性的变化。本文综述了近年来物质表面的浸润性在光刺激下发生转变的研究进展,其中包括无机氧化物表面超疏水和超亲水之间的转换,光响应聚合物表面液滴的运动及接触角的变化,以及光响应聚合物表面黏附性的变化。

关键词： 浸润性, 接触角, 光响应, 超疏水, 超亲水

Surface energy and surface topography are two key factors in the wettability of solid substrates. The surface energy determines the contact angle (CA) of a liquid on a flat substrate and the geometrical factor enhances the wetting property for a hydrophilic surface (or non-wetting for a hydrophobic surface). Applying external stimuli is a valuable approach for rendering the change in surface chemistry and/or topography, and for driving the wettability transition of smart surfaces. This review describes the current state-of-the-art research on the reversibly switchable wettability of surface brought about by external stimuli, including surface conversion between superhydrophobicity and superhydrophilicity prepared from inorganic oxides or/and photoactive organic molecules, movement of liquid droplets driven by molecular machines, and light-driven switching of superhydrophobic adhesion.

Contents
1 Introduction
1.1 Basic theory of surface wettability
1.2 Photoresponsive materials
2 Inorganic-oxide-based photoresponsive surfaces
3 Organic-compound-based photoresponsive surfaces
3.1 Non-azobenzene compound photoresponsive surfaces
3.2 Azobenzene compound photoresponsive surfaces
4 Conclusion

Key words: wetting property, contact angle, photoresponsive, superhydrophobicity, superhydrophilicity

中图分类号: 

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摘要

光响应固体表面的浸润性调控