• 综述与评论 •
王彦斌, 赵红颖, 赵国华, 王宇晶, 杨修春. 基于铁化合物的异相Fenton催化氧化技术[J]. 化学进展, doi: 10.7536/PC121201.
Wang Yanbin, Zhao Hongying, Zhao Guohua, Wang Yujing, Yang Xiuchun. Iron Compound-Based Heterogeneous Fenton Catalytic Oxidation Technology[J]. Progress in Chemistry, doi: 10.7536/PC121201.
异相Fenton催化氧化技术是一种非常有效的处理难生物降解有机污染物的方法,它可以在温和的条件下实现反应。作为均相Fenton的发展,异相Fenton具有容易分离并再利用和更宽的适用范围等优点。该文主要综述了常见的含铁物质作为异相Fenton催化剂降解有机污染物的发展,这些催化剂包括零价铁、氧化铁、羟基氧化铁、水铁矿和其他铁化合物等。全面介绍了Fenton反应的不同机理,包括自由基机理和高价铁机理。重点讨论了提高异相Fenton催化剂活性的发展,并指出催化剂的效率受其表面氧化态、比表面积、过渡金属掺杂种类和晶相等许多因素的影响。概述了提高异相Fenton催化剂催化效率的不同方法,包括减小催化剂尺寸到纳米尺度、将催化剂负载于高比表面积载体上、引入过渡金属(如Ti、Co、Mn、Cr和V)到催化剂结构中。另外,一类新颖的异相Fenton催化剂铁氧体受到特别的关注,这是由于它高的催化活性和稳定性。最后,对异相Fenton催化氧化技术的发展进行了展望。我们认为理想的异相Fenton催化剂要具有高的催化活性和H2O2利用率、良好的稳定性、宽pH应用范围和易于回收利用等特点。
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